Plasmonic Surface Lattice Resonances at the Strong Coupling Regime

被引：274

作者：

Vakevainen, A. I. ^{[1
]}

Moerland, R. J. ^{[1
]}

Rekola, H. T. ^{[1
]}

Eskelinen, A. -P. ^{[1
]}

Martikainen, J. -P. ^{[1
]}

Kim, D. -H. ^{[1
]}

Torma, P. ^{[1
]}

机构：

[1] Aalto Univ, Dept Appl Phys, COMP Ctr Excellence, FI-00076 Aalto, Finland

来源：

NANO LETTERS | 2014年 / 14卷 / 04期

基金：

芬兰科学院;

关键词：

Strong coupling; plasmonics; surface lattice resonance; metal nanoparticle arrays; organic dye molecules; FANO RESONANCES; EXCITONS; PARTICLE; NANOSTRUCTURES; SEMICONDUCTOR; SCATTERING; SYSTEMS; LIGHT;

D O I：

10.1021/nl4035219

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

We show strong coupling involving three different types of resonances in plasmonic nanoarrays: surface lattice resonances (SLRs), localized surface plasmon resonances on single nanoparticles, and excitations of organic dye molecules. The measured transmission spectra show splittings that depend on the molecule concentration. The results are analyzed using finite-difference time-domain simulations, a coupled-dipole approximation, coupled-modes models, and Fano theory. The delocalized nature of the collective SLR modes suggests that in the strong coupling regime molecules near distant nanoparticles are coherently coupled.

引用

页码：1721 / 1727

页数：7

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