Two-photon absorption: an overview of measurements and principles

被引：296
|
作者：
Rumi, Mariacristina [1 ,2 ]
Perry, Joseph W. [1 ,2 ]
机构：
[1] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA
[2] Georgia Inst Technol, Ctr Organ Photon & Elect, Atlanta, GA 30332 USA
来源：
ADVANCES IN OPTICS AND PHOTONICS | 2010年 / 2卷 / 04期
基金：
美国国家科学基金会;
关键词：
CROSS-SECTION MEASUREMENTS; NONLINEAR-OPTICAL PROPERTIES; EXCITED-STATE ABSORPTION; PICOSECOND LASER-PULSES; POWER-SQUARED SENSOR; Z-SCAN MEASUREMENTS; ULTRASHORT-PULSE; ORGANIC-MOLECULES; PHOTOSENSITIZED PRODUCTION; ABSORBING MATERIALS;
D O I：
10.1364/AOP.2.000451
中图分类号：
O43 [光学];
学科分类号：
070207 ; 0803 ;
摘要：
The range of organic compounds whose degenerate two-photon absorption (2PA) spectrum has been reported has increased rapidly in recent years, in parallel with the growing interest in applications based on the 2PA process. The comparison of results from different techniques is not always straightforward, and experimental conditions employed may vary significantly. We overview the concepts underlying 2PA measurements and the common assumptions and approximations used in the data analysis for various techniques. The importance of selecting appropriate excitation regimes under which measurements should be performed and of avoiding contributions from absorption mechanisms in addition to 2PA will be emphasized. (C) 2010 Optical Society of America
引用
收藏
页码：451 / 518
页数：68
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