Two-photon absorption and two-photon induced absorption of liquid toluene at 347.15 nm

被引:5
|
作者
Gong, SH [1 ]
Penzkofer, A [1 ]
机构
[1] Univ Regensburg, Inst Expt & Angew Phys 2, D-93040 Regensburg, Germany
关键词
excited-state absorption; excited-state relaxation; toluene; two-photon absorption; two-photon ionization;
D O I
10.1023/A:1006930612062
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
Pump pulse transmission and time-delayed probe pulse transmission measurements through liquid toluene were performed with linear and circular polarized second harmonic pulses of a mode-locked ruby laser system. Two-photon absorption and two-photon induced absorption are observed. The induced absorption anisotropy is investigated. A theory of two-photon absorption in isotropic media is presented. The two-photon absorption cross-section components, the effective excited-state absorption cross-section, the absorption anisotropy relaxation time and the excited singlet-state relaxation time are determined.
引用
收藏
页码:1145 / 1170
页数:26
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