Construction of MoS2/Tubular-like g-C3N4 Composite Photocatalyst for Improved Visible-Light Photocatalytic Hydrogen Production from Seawater

被引:1
|
作者
Shi Wei-Long [1 ,2 ]
Yang Shuang [1 ]
Wang Jing-Bo [1 ]
Lin Xue [1 ]
Guo Feng [3 ]
Shi Jun-You [1 ]
机构
[1] Beihua Univ, Sch Mat Sci & Engn, Jilin 132013, Jilin, Peoples R China
[2] Jiangsu Univ Sci & Technol, Sch Mat Sci & Engn, Zhenjiang 212003, Jiangsu, Peoples R China
[3] Jiangsu Univ Sci & Technol, Sch Energy & Power, Zhenjiang 212013, Jiangsu, Peoples R China
关键词
photocatalysis; hydrogen production; carbon nitride; molybdenum disulfide; HIGH-CRYSTALLINE G-C3N4; QUANTUM DOTS; HETEROJUNCTION; DEGRADATION; FABRICATION; NANOSHEETS; EVOLUTION; MICRORODS; COCATALYST; COO;
D O I
10.11862/CJIC.2020.168
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
In this work, the development of efficient and stable photocatalyst has been the central topic of scientific research. Herein, MoS2 nanosheets/tubular-likeg-C3N4 (MS/TCN) composite photocatalysts with two dimension/one dimension (2D/1D) nanostructure were fabricated through a facile solvothermal method for photocatalytic hydrogen production from seawater under visible light irradiation, exhibiting enhanced photocatalytic performance in comparison of single MS or TCN. Among of them, MS/TCN-0.5 sample (0.5%(w/w) MoS2) showed optimum H-2 evolution rate of 85.1 mu mol.h(-1) and possessed outstanding stability (no significant decrease after 4 cycles). The enhanced photocatalytic activity of MS/TCN composite photocatalyst can be attributed to the fact that the loading of 2D MS, as a cocatalyst, promotes the transfer of photo - induced electron and improves the separation efficiency of electron - hole pairs of 1D TCN.
引用
收藏
页码:1582 / 1592
页数:11
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