Measurements of thermal-neutron capture cross-section and resonance integral of neptunium-237

被引:5
|
作者
Nakamura, Shoji [1 ]
Kitatani, Fumito [1 ]
Kimura, Atsushi [1 ]
Uehara, Akihiro [2 ,3 ]
Fujii, Toshiyuki [2 ,4 ]
机构
[1] Japan Atom Energy Agcy, Nucl Sci & Engn Directorate, Naka, Ibaraki, Japan
[2] Kyoto Univ, Inst Integral Radiat & Nucl Sience, Kumatori Cho, Osaka, Japan
[3] Natl Inst Quantum & Radiol Sci & Technol, Inage Ku, 4-9-1 Anagawa, Chiba 2638555, Japan
[4] Osaka Univ, 1-1 Yamadaoka, Suita, Osaka 5650871, Japan
关键词
Neptunium-237; Protactinium-233; thermal-neutron capture cross-section; resonance integral; activation method; gamma-ray spectroscopy; emission probability; EMISSION PROBABILITIES; GAMMA-RAYS; NUCLEAR-DATA; DECAY; SPECTRUM; LIBRARY; SCIENCE;
D O I
10.1080/00223131.2019.1598304
中图分类号
TL [原子能技术]; O571 [原子核物理学];
学科分类号
0827 ; 082701 ;
摘要
The thermal-neutron capture cross-section (sigma(0)) and resonance integral (I-0) were measured for the Np-237(n,) Np-238 reaction by an activation method. A method with a Gadolinium filter, which is similar to the Cadmium difference method, was used to measure the sigma(0) with paying attention to the first resonance at 0.489eV of Np-237, and a value of 0.133eV was taken as a cut-off energy. Neptunium-237 samples were irradiated at the pneumatic tube of the Kyoto University Research Reactor in Institute for Integral Radiation and Nuclear Science, Kyoto University. Wires of Co/Al and Au/Al alloys were used as monitors to determine thermal-neutron fluxes and epi-thermal Westcott's indices at an irradiation position. A -ray spectroscopy was used to measure activities of Np-237, Np-238 and neutron monitors. On the basis of Westcott's convention, the sigma(0) and I-0 values were derived as 186.9 +/- 6.2 barn, and 1009 +/- 90 barn, respectively.
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页码:493 / 502
页数:10
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