A review of catalyst modifications for a highly active and stable hydrogen production from methane

被引：14
|
作者：
Gao, Xingyuan [1 ,2 ,3 ]
Wen, Yili [1 ]
Tan, Rui [1 ]
Huang, Haiqing [1 ]
Kawi, Sibudjing [3 ]
机构：
[1] Guangdong Univ Educ, Dept Chem & Mat Sci, Guangzhou 510303, Peoples R China
[2] Engn Technol Dev Ctr Adv Mat & Energy Saving & Emi, Guangzhou 510303, Peoples R China
[3] Natl Univ Singapore, Dept Chem & Biomol Engn, Singapore 117585, Singapore
来源：
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2023年 / 48卷 / 16期
关键词：
Methane; Hydrogen; Reaction mechanism; Catalyst; Deactivation; Anti-deactivation; NI-BASED CATALYSTS; ONE-POT SYNTHESIS; PROMOTED NI/AL2O3 CATALYST; STEAM-REFORMING CATALYSTS; FISCHER-TROPSCH SYNTHESIS; OXIDE FUEL-CELLS; PARTIAL OXIDATION; CARBON-DIOXIDE; NICKEL-CATALYSTS; SYNGAS PRODUCTION;
D O I：
10.1016/j.ijhydene.2022.06.185
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
In the thermo-catalytic hydrogen production from methane, catalyst deactivation is a major issue for the industrial applications. In this review, six modification strategies to achieve a robust catalyst have been discussed in category, including preparation methods, metal-support interaction, support confinement, surface acidity and basicity, oxygen defects and alloys. In addition, the reaction mechanisms of seven methane-involved reactions and three deactivation mechanisms (poisoning, sintering and coking) are illustrated. Moreover, a critical analysis of the synthesis-structure-performance relationship is provided. Finally, conclusive remarks and prospects are proposed. & COPY; 2022 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码：6204 / 6232
页数：29
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