A review of catalyst modifications for a highly active and stable hydrogen production from methane

被引：14

作者：

Gao, Xingyuan ^{[1
,2
,3
]}

Wen, Yili ^{[1
]}

Tan, Rui ^{[1
]}

Huang, Haiqing ^{[1
]}

Kawi, Sibudjing ^{[3
]}

机构：

[1] Guangdong Univ Educ, Dept Chem & Mat Sci, Guangzhou 510303, Peoples R China

[2] Engn Technol Dev Ctr Adv Mat & Energy Saving & Emi, Guangzhou 510303, Peoples R China

[3] Natl Univ Singapore, Dept Chem & Biomol Engn, Singapore 117585, Singapore

来源：

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2023年 / 48卷 / 16期

关键词：

Methane; Hydrogen; Reaction mechanism; Catalyst; Deactivation; Anti-deactivation; NI-BASED CATALYSTS; ONE-POT SYNTHESIS; PROMOTED NI/AL2O3 CATALYST; STEAM-REFORMING CATALYSTS; FISCHER-TROPSCH SYNTHESIS; OXIDE FUEL-CELLS; PARTIAL OXIDATION; CARBON-DIOXIDE; NICKEL-CATALYSTS; SYNGAS PRODUCTION;

D O I：

10.1016/j.ijhydene.2022.06.185

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

In the thermo-catalytic hydrogen production from methane, catalyst deactivation is a major issue for the industrial applications. In this review, six modification strategies to achieve a robust catalyst have been discussed in category, including preparation methods, metal-support interaction, support confinement, surface acidity and basicity, oxygen defects and alloys. In addition, the reaction mechanisms of seven methane-involved reactions and three deactivation mechanisms (poisoning, sintering and coking) are illustrated. Moreover, a critical analysis of the synthesis-structure-performance relationship is provided. Finally, conclusive remarks and prospects are proposed. & COPY; 2022 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

引用

页码：6204 / 6232

页数：29

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