Dual-Driven Functional Fabric with High Electrothermal and Photothermal Conversion Efficiency Modified by CuS Nanoparticles

被引:4
|
作者
Zhang, Jintao [1 ]
Qin, Yajie [1 ]
Pan, Wei [1 ,3 ]
Wang, Zebo [2 ]
Qi, Yu [1 ]
He, Jianxin [1 ]
Zhang, Huiqin [3 ]
机构
[1] Zhongyuan Univ Technol, Int Joint Lab New Text Mat & Text Henan Prov, Zhengzhou 450007, Peoples R China
[2] Zhongyuan Univ Technol, Coll Text, Zhengzhou 451191, Peoples R China
[3] Zhongyuan Univ Technol, Sch Mat & Chem Engn, Zhengzhou 451191, Peoples R China
关键词
polyethylene nanofiber bundles; CuS; electrothermalconversion; photothermal conversion; solar-drivenwater evaporation; COTTON FABRICS; PHOTOCATALYSIS; TEXTILES;
D O I
10.1021/acsapm.3c01047
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
As an ideal substrate for active material integration,fabricsof nanofiber bundles have held great promise due to their outstandingsurface area, unique mechanical flexibility, and textile structure.Herein, a polyethylene nanofiber bundle (PNB) fabric was preparedvia melt blending extrusion followed by chemical deposition of a coppersulfide (CuS) active layer. Benefiting from the high conductivityand the outstanding light absorption characteristics of CuS, CuS/PNBfabrics exhibited excellent photo and electric dual-driven energyconversion performance. Specifically, the CuS/PNB fabrics showed thehighest electrical conductivity (277 S m(-1)), exceptionalJoule heating (up to 85.7 & DEG;C at a voltage of 0.8 V), a low workingvoltage (0.2-0.8 V), and long-term stability. Furthermore,the photo-absorption efficiency and surface temperature reached 94.3%and 91.2 & DEG;C under the irradiation of 1 sun, respectively. Meanwhile,the CuS/PNB fabrics exhibited a high specific evaporation rate ofup to 1.81 kg m(-2) h(-1), as wellas an energy conversion efficiency of 95.1% under one solar irradiation.We believe that such a functional fabric offers a strategy for energyharvesting and conversion fields and displays promising applicationsin warmth-keeping and solar-driven water evaporation in the future.
引用
收藏
页码:5747 / 5757
页数:11
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