Enhanced diffusion of tracer particles in nonreciprocal mixtures

被引:5
|
作者
Benois, Anthony [1 ]
Jardat, Marie [1 ]
Dahirel, Vincent [1 ]
Demery, Vincent [2 ,3 ]
Agudo-Canalejo, Jaime [4 ]
Golestanian, Ramin [4 ,5 ]
Illien, Pierre [1 ]
机构
[1] Sorbonne Univ, CNRS, Phys Chim Electrolytes & Nanosyst Interfaciaux PHE, F-75005 Paris, France
[2] ESPCI Paris PSL, Gulliver, CNRS, UMR 7083, F-75005 Paris, France
[3] Univ Claude Bernard, Univ Lyon, ENS Lyon, CNRS, F-69342 Lyon, France
[4] Max Planck Inst Dynam & Selforg, Dept Living Matter Phys, D-37077 Gottingen, Germany
[5] Univ Oxford, Rudolf Peierls Ctr Theoret Phys, Oxford OX1 3PU, England
关键词
FLUID;
D O I
10.1103/PhysRevE.108.054606
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
We study the diffusivity of a tagged particle in a binary mixture of Brownian particles with nonreciprocal interactions. Numerical simulations reveal that, for a broad class of interaction potentials, nonreciprocity can significantly increase the long-time diffusion coefficient of tracer particles and that this diffusion enhancement is associated with a breakdown of the Einstein relation. These observations are quantified and confirmed via two different and complementary analytical approaches: (i) a linearized stochastic density field theory, which is particularly accurate in the limit of soft interactions, and (ii) a reduced two-body description, which is exact at leading order in the density of particles. The latter reveals that diffusion enhancement can be attributed to the formation of transiently propelled dimers of particles, whose cohesion and speed are controlled by the nonreciprocal interactions.
引用
收藏
页数:14
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