Direct Air Carbon Capture and Recovery Utilizing Alkaline Solution Circulation

被引:5
|
作者
Liu, Lishan [1 ]
Gong, Feng [1 ]
Xiao, Rui [1 ]
机构
[1] Southeast Univ, Sch Energy & Environm, Key Lab Energy Thermal Convers & Control, Minist Educ, Nanjing 210096, Peoples R China
基金
中国国家自然科学基金;
关键词
CO2; ENERGY;
D O I
10.1021/acs.energyfuels.3c01296
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
Direct air capture (DAC) represents a promising technologyformitigating climate change by extracting CO2 from the atmosphere.This study introduces a novel application for effective CO2 capture from dispersed emission sources, integrated with a liquidelectrolysis system to improve capture cycle efficiency. By focusingon distributed sources, the DAC application overcomes the constraintsof traditional stationary CO2 capture methods. It employsa thin-layer moving bed spray and air convection to capture CO2 in lean liquid, which converts into rich trap liquid whenthe carbonate concentration exceeds a certain threshold. Electrolysisis then used to recover the lean liquid. This design allows for quick,energy-efficient CO2 absorption even under low partialpressure conditions (462 ppm). The technology is designed to facilitatesignificant CO2 capture while concurrently generating high-purityhydrogen and collecting carbon dioxide. By reusing the capture liquid,an integrated capture and desorption process is realized. In a testwith 1 M KOH as a lean trap solution and a wind speed of 9 m/s, arich trap solution was obtained after 13 h, lowering the CO2 concentration at the outlet by 97 ppm compared to the input air,demonstrating the device's effectiveness.
引用
收藏
页码:9339 / 9346
页数:8
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