Stable and easily detachable cellulose-based membrane system inspired by water hyacinth for efficient heavy metals removal from water

被引:0
|
作者
Zhang, Fang [1 ,2 ]
Sun, Yuxin [1 ]
Qian, Xinye [1 ]
Tan, Xiaoyan [1 ]
Liu, Peipei [1 ]
Yao, Zhong [1 ]
Zheng, Chunling [1 ,2 ,3 ]
Hu, Yonghong [1 ,2 ]
机构
[1] Nanjing Tech Univ, Coll Food Sci & Light Ind, Nanjing 211800, Jiangsu, Peoples R China
[2] State Key Lab Mat Oriented Chem Engn, Nanjing 211800, Jiangsu, Peoples R China
[3] Nanjing Tech Univ, Inst Text Chem & Ecol Dyeing & Finishing, Nanjing 211800, Jiangsu, Peoples R China
关键词
Biomimetic membrane; Cellulose/lignin microdevice; Heavy metal ions; Extraction and enrichment; HIGH LOADINGS; ADSORPTION; AEROGEL; WASTE; ACID;
D O I
10.1007/s10570-023-05579-w
中图分类号
TB3 [工程材料学]; TS [轻工业、手工业、生活服务业];
学科分类号
0805 ; 080502 ; 0822 ;
摘要
membrane phase and finally locked in the NLMD, as demonstrated by extraction efficiency (3 min, similar to 90%), as well as high-enrichment (similar to 27 times) toward Pb, Zn, and Cu ions. The NLMD was fabricated using nanocellulose and reinforced using lignin-polyamide epoxy chloropropane nanoaggregates that endow the high mechanical stability and good W/O interfacial affinity of the NLMD. Significantly, the BMS could be facilely detached via simple filtration and shape recovery, offering a high-performance and facile regeneration pathway that are hardly attainable by the conventional cellulose-based adsorbents.A rapid extracted and concentrated system engineered by green polymers is attractive but there is still a challenge with respect to both materials and processes. Water hyacinth root cells have evolved as a biological membrane system that can transport and concentrate metal ions from water to the plant body rather than simply utilizing the intrinsic trapping properties of cellulose/lignin. This has inspired a novel biological membrane system (BMS), namely, a porous nanocellulose/lignin microdevice (NLMD) accommodated with a stripping agent that is dispersed in an organic phase. In practice, in water, metal ions can be efficiently transported through an organic
引用
收藏
页码:11619 / 11632
页数:14
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