Rapid and stable hydrogen detection based on Pd-modified WO3 nanosheets

被引:2
|
作者
Lv, Jianxin [1 ]
Zhang, Linghui [1 ]
Si, Lianxi [3 ]
Li, Hui [1 ,2 ]
Zhao, Wenbo [1 ]
An, Fei [4 ]
Feng, Xia [1 ]
Hu, Shi [1 ,2 ]
机构
[1] Tianjin Univ, Sch Sci, Dept Chem, Tianjin Key Lab Mol Optoelect Sci, Tianjin 300072, Peoples R China
[2] Inst Energy, Hefei Comprehens Natl Sci Ctr, Hefei 230000, Anhui, Peoples R China
[3] Tianjin Univ, Sch Chem Engn & Technol, Tianjin 300072, Peoples R China
[4] SINOPEC Res Inst Safety Engn Co Ltd, State Key Lab Safety & Control Chem, Songling Rd 339, Qingdao 266000, Shandong, Peoples R China
基金
中国国家自然科学基金;
关键词
MESOPOROUS WO3; THIN-FILMS; NANOPARTICLES; SEMICONDUCTOR; SENSITIZATION; PERFORMANCE; DEPOSITION; CATALYSTS; ANGLE;
D O I
10.1039/d3dt00338h
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
Materials with accurate and durable gas detection are essential for gas sensors. We developed a facile and effective method to deposit Pd onto WO3 nanosheets and used the samples for hydrogen gas sensing. The combination of the 2D ultrathin nanostructure of WO3 and the spillover effect of Pd enables a detection concentration down to 20 ppm of hydrogen and high selectivity against other gases including methane, butane, acetone, isopropanol, etc. Moreover, the durability of the sensing materials was testified through 50 cycles of exposure to 200 ppm of hydrogen. These outstanding performances are mainly attributed to a homogeneous and tenacious decoration of Pd on the surface of WO3 nanosheets, providing an attractive choice for practical applications.
引用
收藏
页码:4200 / 4206
页数:7
相关论文
共 50 条
  • [1] SAW hydrogen gas sensor based on WO3 and Pd nanostructures
    Jakubik, Wieslaw
    Urbanczyk, Marian
    Maciak, Erwin
    [J]. PROCEEDINGS OF THE EUROSENSORS XXIII CONFERENCE, 2009, 1 (01): : 200 - 203
  • [2] Investigations of thin film structures of WO3 and WO3 with Pd for hydrogen detection in a surface acoustic wave sensor system
    Jakubik, W. P.
    [J]. THIN SOLID FILMS, 2007, 515 (23) : 8345 - 8350
  • [3] Preparation of a Pd membrane on a WO3 modified Porous Stainless Steel for hydrogen separation
    Zahedi, Mostafa
    Afra, Boshra
    Dehghani-Mobarake, Mostafa
    Bahmani, Majid
    [J]. JOURNAL OF MEMBRANE SCIENCE, 2009, 333 (1-2) : 45 - 49
  • [4] Surface AcousticWave Hydrogen Sensors Based on Nanostructured Pd/WO3 Bilayers
    Miu, Dana
    Birjega, Ruxandra
    Viespe, Cristian
    [J]. SENSORS, 2018, 18 (11)
  • [5] Hydrogen sensors based on 2D WO3 nanosheets prepared by anodization
    Rahmani, Mohammad Bagher
    Yaacob, Mohd Hanif
    Sabri, Ylias Mohammad
    [J]. SENSORS AND ACTUATORS B-CHEMICAL, 2017, 251 : 57 - 64
  • [6] 2-D WO3 decorated with Pd for rapid gasochromic and electrical hydrogen sensing
    Kalanur, Shankara S.
    Heo, Jaewoo
    Yoo, Il-Han
    Seo, Hyungtak
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2017, 42 (26) : 16901 - 16908
  • [7] MoS2/WO3 Nanosheets for Detection of Ammonia
    Singh, Sukhwinder
    Deb, Jyotirmoy
    Sarkar, Utpal
    Sharma, Sandeep
    [J]. ACS APPLIED NANO MATERIALS, 2021, 4 (03) : 2594 - 2605
  • [8] Fabrication of Pd Doped WO3 Nanofiber as Hydrogen Sensor
    Nikfarjam, Alireza
    Fardindoost, Somayeh
    Zad, Azam Iraji
    [J]. POLYMERS, 2013, 5 (01) : 45 - 55
  • [9] Hydrogen Sensing Properties of WO3/Pd composite films
    Li, Jinhua
    Zhao, Meng
    Su, Jiangbin
    Jiang, Meiping
    [J]. APPLICATIONS OF ENGINEERING MATERIALS, PTS 1-4, 2011, 287-290 : 2343 - +
  • [10] Hydrogen sensing mechanism of Ru-loaded WO3 nanosheets
    Huang, Dan
    Yuan, Wenjing
    Fan, Shurui
    Tian, Chen
    Hua, Zhongqiu
    Tian, Xuemin
    Wu, Yi
    Li, Er-ping
    [J]. SENSORS AND ACTUATORS B-CHEMICAL, 2020, 304