Synthesis and assembly of two-dimensional heterostructured architectures

被引：1

作者：

Flouda, Paraskevi ^{[1
]}

Choi, Jinyoung ^{[1
]}

Buxton, Madeline L. L. ^{[1
]}

Nepal, Dhriti ^{[2
]}

Lin, Zhiqun ^{[1
,3
]}

Bunning, Timothy J. J. ^{[2
]}

Tsukruk, Vladimir V. V. ^{[1
]}

机构：

[1] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA

[2] Wright Patterson AFB Res Lab, Mat & Mfg Directorate, Wright, OH 45433 USA

[3] Natl Univ Singapore, Dept Chem & Biomol Engn, Singapore 117585, Singapore

来源：

MRS COMMUNICATIONS | 2023年 / 13卷 / 05期

基金：

美国国家科学基金会;

关键词：

2D materials; Atomic probe microscopy; Chemical synthesis; Heterogeneous heterostructure; Nanostructure; Self-assembly of heterostructures; GRAPHENE-BASED MATERIALS; 2D TITANIUM CARBIDE; PSEUDOCAPACITIVE ELECTRODES; BATTERY APPLICATIONS; MXENE NANOSHEETS; TI3C2TX MXENE; OXIDE; CONVERSION; NANOSTRUCTURES; POLYMERIZATION;

D O I：

10.1557/s43579-023-00412-8

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

Stacking atomically thin two-dimensional nanosheet materials leads to unique synergy in their inherent properties due to an intimate combination and matching that is not possible via separate individual components and phases. However, traditional synthesis and assembly methods result in poor architectural control, diffuse interfaces and restricted surface chemistry, thereby limiting their prospective potentials. This brief overview provides condensed consideration of different synthesis and assembly methods for the fabrication of diverse novel heterostructures from individual nanosheets and challenges of existing methods. Finally, future perspectives regarding crafting of well-defined heterostructures with highly controllable architectures and interfacial/surface chemistry and advanced characterization methods are highlighted.

引用

页码：674 / 684

页数：11

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