Magnetic and electronic properties unveil polaron formation in Eu5In2Sb6

被引:0
|
作者
Crivillero, M. Victoria Ale [1 ]
Roessler, Sahana [1 ]
Doerr, M. [2 ]
Granovsky, S. [2 ]
Cook, M. S. [3 ]
Rosa, Priscila F. S. [3 ]
Mueller, J. [4 ]
Wirth, S. [1 ]
机构
[1] Max Planck Inst Chem Phys Solids, Nothnitzer Str 40, D-01187 Dresden, Germany
[2] Tech Univ Dresden, Inst Solid State & Mat Phys, D-01062 Dresden, Germany
[3] Los Alamos Natl Lab, Los Alamos, NM 87545 USA
[4] Goethe Univ Frankfurt, Inst Phys, D-60438 Frankfurt, Germany
来源
SCIENTIFIC REPORTS | 2023年 / 13卷 / 01期
关键词
ZINTL PHASES; EU; MAGNETORESISTANCE; TRANSITION; ORDER; AL;
D O I
10.1038/s41598-023-28711-z
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
The intermetallic compound Eu5In2Sb6, an antiferromagnetic material with nonsymmorphic crystalline structure, is investigated by magnetic, electronic transport and specific heat measurements. Being a Zintl phase, insulating behavior is expected. Our thermodynamic and magnetotransport measurements along different crystallographic directions strongly indicate polaron formation well above the magnetic ordering temperatures. Pronounced anisotropies of the magnetic and transport properties even above the magnetic ordering temperature are observed despite the Eu2+ configuration which testify to complex and competing magnetic interactions between these ions and give rise to intricate phase diagrams discussed in detail. Our results provide a comprehensive framework for further detailed study of this multifaceted compound with possible nontrivial topology.
引用
收藏
页数:9
相关论文
共 50 条
  • [21] Structure, magnetic, opto-electronic and thermoelectric properties of A3In2As4 and A5In2As6 (A = Sr and Eu) Zintl phase compounds
    Taha, T. A.
    Mehmood, Shahid
    Ali, Zahid
    Khan, ShahRukh
    Aman, Salma
    Farid, Hafiz Muhammad Tahir
    Trukhanov, S. V.
    Zubar, T. I.
    Tishkevich, D. I.
    Trukhanov, A. V.
    JOURNAL OF ALLOYS AND COMPOUNDS, 2023, 938
  • [22] Electronic, optical, and magnetic properties of LiFePO4:: Small magnetic polaron effects
    Zaghib, K.
    Mauger, A.
    Goodenough, J. B.
    Gendron, F.
    Julien, C. M.
    CHEMISTRY OF MATERIALS, 2007, 19 (15) : 3740 - 3747
  • [23] Magnetic and magnetocaloric properties of Tb5Si2Sb2
    Nirmala, R.
    Nigam, A. K.
    Malik, S. K.
    SOLID STATE COMMUNICATIONS, 2008, 146 (3-4) : 121 - 123
  • [24] Electronic structure and magnetic properties of β-Ti6Sn5
    Jeong, T.
    JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS, 2007, 309 (01) : 71 - 74
  • [25] Structure and magnetic properties of Eu2CaCu2O6
    Xu, Qiang
    Klimczuk, Tomasz
    Jansen, Jacob
    Cava, Robert J.
    Zandbergen, Henny W.
    CHEMISTRY OF MATERIALS, 2006, 18 (19) : 4585 - 4591
  • [26] 2-SITE POLARON PROBLEM - ELECTRONIC AND VIBRATIONAL PROPERTIES
    RANNINGER, J
    THIBBLIN, U
    PHYSICAL REVIEW B, 1992, 45 (14): : 7730 - 7738
  • [27] Electronic structure, polaron formation, and functional properties in transition-metal tungstates
    Hoang, Khang
    Oh, Myungkeun
    Choi, Yongki
    RSC ADVANCES, 2018, 8 (08) : 4191 - 4196
  • [28] Crystal structure and magnetic properties of the compound FeDY6Sb2
    Zeng, Lingmin
    Qin, Pingli
    Qin, Haiqing
    Zhang, Jiliang
    MATERIALS LETTERS, 2007, 61 (01) : 300 - 303
  • [29] Electronic structures and optical properties of GeTe and Ge2Sb2Te5
    Yamanaka, S
    Ogawa, S
    Morimoto, I
    Ueshima, Y
    JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS SHORT NOTES & REVIEW PAPERS, 1998, 37 (6A): : 3327 - 3333
  • [30] Electronic properties of amorphous and crystalline Ge2Sb2Te5 films
    Kato, T
    Tanaka, K
    JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS BRIEF COMMUNICATIONS & REVIEW PAPERS, 2005, 44 (10): : 7340 - 7344