Fabrication of micro/nano wettability MoS2 hydrogen evolution electrocatalyst based on femtosecond laser

被引:1
|
作者
Wang, Zekun [1 ]
Song, Lin [1 ]
Tao, Haiyan [1 ,3 ]
He, Yaowen [1 ]
Yang, Ying [2 ]
Wang, Tianqi [2 ]
Yu, Hui [2 ]
Lin, Jingquan [1 ,3 ]
Dong, Xiangting [2 ]
机构
[1] Changchun Univ Sci & Technol, Sch Phys, Changchun 130022, Peoples R China
[2] Changchun Univ Sci & Technol, Key Lab Appl Chem & Nanotechnol Univ Jilin Prov, Changchun 130022, Peoples R China
[3] Changchun Univ Sci & Technol, Zhongshan Inst, Zhongshan 528637, Peoples R China
基金
中国国家自然科学基金;
关键词
Femtosecond laser; Superaerophobic electrodes; Micro-/nano-structure; Hydrogen evolution; MoS2; EFFICIENT; CATALYSTS; STRATEGY;
D O I
10.1016/j.ijhydene.2023.08.160
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The process of hydrogen production through water electrolysis involves ionic interactions and the dynamic process of hydrogen bubble formation on the electrode surface. In this study, we employed a combination of femtosecond laser and hydrothermal synthesis to fabricate a novel MoS2 electrode. The double-scale structure of this substrate increases its specific surface area, facilitating the presence of active sites for the hydrogen evolution reaction. The growth of nano-scale catalyst further enhances wettability, promoting rapid detachment of gas bubbles and replenishment of water. This method not only facilitates ionic interactions but also accelerates the formation of macroscopic bubbles. Under alkaline conditions, electrode achieved an impressive current density of 10 mA cm-2 with a low overpotential of only 99 mV. This novel MoS2 hydrogen evolution catalyst holds practical value, paving the way for the design of more efficient and stable electrocatalysts.(c) 2023 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:327 / 335
页数:9
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