Mode-coupling theory for the dynamics of dense underdamped active Brownian particle system

被引:4
|
作者
Feng, Mengkai [1 ,2 ]
Hou, Zhonghuai [1 ,2 ]
机构
[1] Univ Sci & Technol China, Hefei Natl Res Ctr Phys Sci Microscale, Anhui 230026, Peoples R China
[2] Univ Sci & Technol China, Dept Chem Phys, Hefei 230026, Anhui, Peoples R China
来源
JOURNAL OF CHEMICAL PHYSICS | 2023年 / 158卷 / 02期
关键词
GLASS-TRANSITION; SUPERCOOLED LIQUIDS;
D O I
10.1063/5.0131080
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We present a theory to study the inertial effect on glassy dynamics of the underdamped active Brownian particle (UABP) system. Using the assumption of the nonequilibrium steady-state, we obtain an effective Fokker-Planck equation for the probability distribution function (PDF) as a function of positions and momentums. With this equation, we achieve the evolution equation of the intermediate scattering function through the Zwanzig-Mori projection operator method and the mode-coupling theory (MCT). Theoretical analysis shows that the inertia of the particle affects the memory function and corresponding glass transition by influencing the structure factor and a velocity correlation function. The theory provides theoretical support and guidance for subsequent simulation work.
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页数:14
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