Ultra-flexible Al2O3 fibers: A novel catalyst support material for sustainable catalysis

被引:2
|
作者
Yan, Huihui [1 ]
Wang, Kun [1 ]
Zhao, Liping [1 ]
Zhang, Peng [1 ]
Liu, Jing [1 ]
Gao, Lian [1 ]
机构
[1] Shanghai Jiao Tong Univ, Sch Mat Sci & Engn, State Key Lab Met Matrix Composite Mat, Shanghai 200240, Peoples R China
基金
中国国家自然科学基金;
关键词
Inorganic fibers; Flexible fibers; Al; 2; O; 3; fibers; Catalysts; CERAMIC AEROGELS; NANOFIBERS; FABRICATION; RESISTANT;
D O I
10.1016/j.ceramint.2023.06.283
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Flexible aluminum oxide (Al2O3) fibers were prepared by the blow spinning method and their potential as a high temperature catalyst support was investigated. The synthesized Al2O3 fibers exhibited remarkable flexibility in both mechanical compression and recovery tests, which remained intact in a wide temperature range from-196 degrees C to 1200 degrees C. Moreover, their low thermal conductivity of 0.030 W K1 center dot m- 1,demonstrated an outstanding thermal insulation. Subsequently, nickel nanoparticles were uniformly distributed on the surface of the Al2O3 fibers as a self-supporting catalyst using a conventional impregnation method. The resulting selfsupporting Ni/Al2O3 catalyst demonstrated remarkable thermo-catalytic performance and re-activation capability at high temperatures for thermocatalytic reaction of dry reforming of methane (DRM). Our findings highlight the potential of pure Al2O3 flexible fibers as a versatile material for various industrial applications, including high-temperature catalysis.
引用
收藏
页码:30257 / 30265
页数:9
相关论文
共 50 条
  • [31] Transparent and flexible capacitors based on nanolaminate Al2O3/TiO2/Al2O3
    Zhang, Guozhen
    Wu, Hao
    Chen, Chao
    Wang, Ti
    Yue, Jin
    Liu, Chang
    NANOSCALE RESEARCH LETTERS, 2015, 10
  • [32] A novel catalyst for hydrazine decomposition:: molybdenum carbide supported on γ-Al2O3
    Chen, XW
    Zhang, T
    Ying, PL
    Zheng, MY
    Wu, WC
    Xia, LG
    Li, T
    Wang, XD
    Li, C
    CHEMICAL COMMUNICATIONS, 2002, (03) : 288 - 289
  • [33] MoP/Al2O3 as a novel catalyst for sulfur-resistant methanation
    Wang, Baowei
    Zhao, Jun
    Meng, Dajun
    Li, Zhenhua
    Xu, Yan
    Ma, Xinbin
    APPLIED ORGANOMETALLIC CHEMISTRY, 2018, 32 (10)
  • [34] PREPARATION OF NOVEL Pd/γ-Al2O3 NANOFIBRE NONWOVEN BASED CATALYST
    Wei-min, Kang
    Bo-wen, Cheng
    Quan-xiang, Li
    86TH TEXTILE INSTITUTE WORLD CONFERENCE, VOL 4, CONFERENCE PROCEEDINGS, 2008, : 2293 - 2302
  • [35] Sol-gel Ni/γ-Al2O3 material as secondary catalyst for toluene reforming: Tailoring the γ-Al2O3 substrate with stearic acid
    Claude, Vincent
    Mahy, Julien G.
    Micheli, Francesca
    Geens, Jeremy
    Lambert, Stephanie D.
    MICROPOROUS AND MESOPOROUS MATERIALS, 2020, 291 (291)
  • [36] Improved performance of Ni/Al2O3 catalyst deriving from the hydrotalcite precursor synthesized on Al2O3 support for dry reforming of methane
    Xu, Yan
    Du, Xihua
    Shi, Liluo
    Chen, Teng
    Wan, Hongri
    Wang, Peng
    Wei, Shuai
    Yao, Bing
    Zhu, Jie
    Song, Ming
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2021, 46 (27) : 14301 - 14310
  • [37] The effect of chlorine and support dissolution on hydrogen chemisorption on Ru/Al2O3 Catalyst
    Okal, J.
    POLISH JOURNAL OF CHEMISTRY, 2007, 81 (01) : 69 - 77
  • [38] OPTIMIZATION OF REFORMING CATALYST SUPPORT (AL2O3) IN SPHERICAL SHAPE MANUFACTURE CONDITIONS
    RADOMYSKI, B
    SZCZYGIEL, J
    MARCINKOWSKI, M
    PRZEMYSL CHEMICZNY, 1986, 65 (07): : 352 - 354
  • [39] Influence of calcination temperature on the structure and properties of Al2O3 as support for Pd catalyst
    Mi Yeon Byun
    Ji Sun Kim
    Dae-Won Park
    Man Sig Lee
    Korean Journal of Chemical Engineering, 2018, 35 : 1083 - 1088
  • [40] Hydrogen adsorbed species at the metal/support interface on a Pt/Al2O3 catalyst
    FerreiraAparicio, P
    GuerreroRuiz, A
    RodriguezRamos, I
    JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS, 1997, 93 (19): : 3563 - 3567