Bioelectrocatalytic Synthesis: Concepts and Applications

被引：25

作者：

Boucher, Dylan G. ^{[1
]}

Carroll, Emily ^{[1
]}

Nguyen, Zachary A. ^{[1
]}

Jadhav, Rohit G. ^{[1
]}

Simoska, Olja ^{[2
]}

Beaver, Kevin ^{[1
]}

Minteer, Shelley D. ^{[1
]}

机构：

[1] Univ Utah, Dept Chem, Salt Lake City, UT 84112 USA

[2] Univ South Carolina, Dept Chem & Biochem, Columbia, SC 29208 USA

来源：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2023年 / 62卷 / 46期

关键词：

Biocatalysis; Bioelectrochemistry; Electrocatalysis; Electrochemistry; Electrosynthesis; EXTRACELLULAR ELECTRON-TRANSFER; NANOWIRE-BACTERIA HYBRIDS; MICROBIAL ELECTROSYNTHESIS; CARBON-DIOXIDE; ENZYMATIC ELECTROSYNTHESIS; ELECTROENZYMATIC REDUCTION; ELECTRICITY PRODUCTION; REDUCING BACTERIUM; NITROGEN-FIXATION; ESCHERICHIA-COLI;

D O I：

10.1002/anie.202307780

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Bioelectrocatalytic synthesis is the conversion of electrical energy into value-added products using biocatalysts. These methods merge the specificity and selectivity of biocatalysis and energy-related electrocatalysis to address challenges in the sustainable synthesis of pharmaceuticals, commodity chemicals, fuels, feedstocks and fertilizers. However, the specialized experimental setups and domain knowledge for bioelectrocatalysis pose a significant barrier to adoption. This review introduces key concepts of bioelectrosynthetic systems. We provide a tutorial on the methods of biocatalyst utilization, the setup of bioelectrosynthetic cells, and the analytical methods for assessing bioelectrocatalysts. Key applications of bioelectrosynthesis in ammonia production and small-molecule synthesis are outlined for both enzymatic and microbial systems. This review serves as a necessary introduction and resource for the non-specialist interested in bioelectrosynthetic research.

引用

页数：32

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