Identification of volatile organic compound emissions from anthropogenic and biogenic sources based on satellite observation of formaldehyde and glyoxal

被引:7
|
作者
Chen, Yujia [1 ]
Liu, Cheng [1 ,2 ,3 ,4 ,5 ]
Su, Wenjing [6 ,7 ]
Hu, Qihou [1 ]
Zhang, Chengxin [2 ]
Liu, Haoran [8 ]
Yin, Hao [1 ]
机构
[1] Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Key Lab Environm Opt & Technol, Hefei 230031, Peoples R China
[2] Univ Sci & Technol China, Dept Precis Machinery & Precis Instrumentat, Hefei 230026, Peoples R China
[3] Chinese Acad Sci, Ctr Excellence Reg Atmospher Environm, Inst Urban Environm, Xiamen 361021, Peoples R China
[4] Univ Sci & Technol China, Key Lab Precis Sci Instrumentat, Anhui Higher Educ Inst, Hefei 230026, Peoples R China
[5] Univ Sci & Technol China, Anhui Prov Key Lab Polar Environm & Global Change, Hefei 230026, Peoples R China
[6] Univ Sci & Technol China, Dept Environm Sci & Engn, Hefei 230026, Peoples R China
[7] China Meteorol Adm, Key Lab Atmospher Chem, Beijing 100089, Peoples R China
[8] Anhui Univ, Inst Phys Sci & Informat Technol, Hefei 230601, Peoples R China
基金
中国国家自然科学基金;
关键词
Volatile organic compounds; Ratio of glyoxal and formaldehyde; TROPOMI; Anthropogenic emission; SENTINEL-5; PRECURSOR; RIVER DELTA; GLOBAL OBSERVATIONS; SECONDARY SOURCES; AIR-QUALITY; LIGHT-DUTY; TROPOMI; TRENDS; COLUMNS; CHINA;
D O I
10.1016/j.scitotenv.2022.159997
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Anthropogenic volatile organic compounds (VOCs) are serious pollutants in the atmosphere because of their toxicity and as precursors of secondary organic aerosols and ozone pollution. Although in-situ measurements provide accurate information on VOCs, their spatial coverage is limited and insufficient. In this study, we provide a global perspective for identifying anthropogenic VOC emission sources through the ratio of glyoxal to formaldehyde (RGF) based on satellite observations. We assessed typical cities and polluted areas in the mid latitudes and found that some Asian cities had higher anthropogenic VOC emissions than cities in Europe and America. For heavily polluted areas, such as the Yangtze River Delta (YRD), the areas dominated by anthropogenic VOCs accounted for 23 % of the total study areas. During the COVID-19 pandemic, a significant decline in RGF values was observed in the YRD and western United States, corresponding to a reduction in anthropogenic VOC emissions. Furthermore, developing countries appeared to have higher anthropogenic VOC emissions than developed countries. These observations could contribute to optimising industrial structures and setting stricter pollution standards to reduce anthropogenic VOCs in developing countries.
引用
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页数:12
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