Regulating the Pt1-CeO2 interaction via alkali modification for boosting the catalytic performance of single-atom catalysts

被引:7
|
作者
Yang, Peng [1 ,2 ,3 ]
Xu, Juntian [1 ,2 ,3 ]
Tan, Wei [1 ,2 ,3 ]
Liu, Qinglong [1 ,2 ,3 ]
Cai, Yandi [1 ,2 ,3 ]
Xie, Shaohua [4 ]
Hong, Song [5 ]
Gao, Fei [1 ,2 ,3 ]
Liu, Fudong [4 ]
Dong, Lin [1 ,2 ,3 ]
机构
[1] Nanjing Univ, Sch Environm, State Key Lab Pollut Control & Resource Reuse, Nanjing 210023, Peoples R China
[2] Nanjing Univ, Ctr Modern Anal, Jiangsu Key Lab Vehicle Emiss Control, Nanjing 210023, Peoples R China
[3] Nanjing Univ, Sch Chem & Chem Engn, Key Lab Mesoscop Chem MOE, Nanjing 210023, Peoples R China
[4] Univ Cent Florida, Nanosci Technol Ctr NSTC, Catalysis Cluster Renewable Energy & Chem Transfor, Dept Civil Environm & Construction Engn, Orlando, FL 32816 USA
[5] Beijing Univ Chem Technol, Coll Mat Sci & Engn, Beijing 100029, Peoples R China
基金
中国国家自然科学基金;
关键词
TEMPERATURE; SUPPORT; CEO2;
D O I
10.1039/d3cc00387f
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
With the introduction of potassium species, the catalytic oxidation performance over the Pt-1/CeO2 catalyst was significantly enhanced, where potassium ions acted as structural and electronic promoters, and formed Pt-O-K interactions with Pt to directly regulate the coordination environment and electronic state of Pt and the metal-support interaction between Pt and CeO2.
引用
收藏
页码:6219 / 6222
页数:4
相关论文
共 50 条
  • [21] Modulating the local coordination environment of single-atom catalysts for enhanced catalytic performance
    Li, Xinyuan
    Rong, Hongpan
    Zhang, Jiatao
    Wang, Dingsheng
    Li, Yadong
    NANO RESEARCH, 2020, 13 (07) : 1842 - 1855
  • [22] Modulating the local coordination environment of single-atom catalysts for enhanced catalytic performance
    Xinyuan Li
    Hongpan Rong
    Jiatao Zhang
    Dingsheng Wang
    Yadong Li
    Nano Research, 2020, 13 : 1842 - 1855
  • [23] Photothermal Synergistic Effect of Pt1/CuO-CeO2 Single-Atom Catalysts Significantly Improving Toluene Removal
    Feng, Ying
    Dai, Lingyun
    Wang, Zhiwei
    Peng, Yue
    Duan, Erhong
    Liu, Yuxi
    Jing, Lin
    Wang, Xun
    Rastegarpanah, Ali
    Dai, Hongxing
    Deng, Jiguang
    ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2022, 56 (12) : 8722 - 8732
  • [24] Single-atom catalysts in the catalytic production of H2O2
    Li, Zhiqi
    Yu, Zhihan
    Guan, Chen
    Xu, Kaiqiang
    Xiang, Quanjun
    JOURNAL OF MATERIOMICS, 2025, 11 (04)
  • [25] Influence of Local Chemical Environment on the Catalytic Properties of Ir1/CeO2 Single-Atom Catalysts in CO Oxidation
    Pauletti, Carlo Federico
    Camellone, Matteo Farnesi
    Piccinin, Simone
    ACS CATALYSIS, 2025, 15 (07): : 5806 - 5824
  • [26] Electronic Regulation of Pt Single-Atom Catalysts via Local Coordination State Adjustment for Enhanced Photocatalytic Performance
    Zhai, Huanhuan
    Tan, Pengfei
    Jiang, Min
    Zhang, Mingyuan
    Ren, Ruifeng
    Sa, Rongjian
    Pan, Jun
    ACS CATALYSIS, 2023, 13 (12) : 8063 - 8072
  • [27] Regulating the coordination microenvironment of zinc single-atom catalysts to enhance intramolecular hydroamination performance
    Wang, Li
    Lv, Chao
    Dou, Kecan
    Xie, Deqiong
    Fu, Yanghe
    Zhang, Fumin
    Chen, De-Li
    Zhu, Weidong
    INORGANIC CHEMISTRY FRONTIERS, 2024, 11 (14): : 4207 - 4218
  • [28] Mass production of thermally stable Pt single-atom catalysts for the catalytic oxidation of sulfur dioxide
    Jianchen, Wang
    Yong, Kang
    Sun, Fangkuan
    Catalysis Science and Technology, 2022, 12 (01): : 124 - 134
  • [29] A tailored oxide interface creates dense Pt single-atom catalysts with high catalytic activity
    Yoo, Mi
    Yu, Young-Sang
    Ha, Hyunwoo
    Lee, Siwon
    Choi, Jin-Seok
    Oh, Sunyoung
    Kang, Eunji
    Choi, Hyuk
    An, Hyesung
    Lee, Kug-Seung
    Park, Jeong Young
    Celestre, Richard
    Marcus, Matthew A.
    Nowrouzi, Kasra
    Taube, Doug
    Shapiro, David A.
    Jung, WooChul
    Kim, Chunjoong
    Kim, Hyun You
    ENERGY & ENVIRONMENTAL SCIENCE, 2020, 13 (04) : 1231 - 1239
  • [30] Mass production of thermally stable Pt single-atom catalysts for the catalytic oxidation of sulfur dioxide
    Wang Jianchen
    Kang Yong
    Sun, Fangkuan
    CATALYSIS SCIENCE & TECHNOLOGY, 2022, 12 (01) : 124 - 134