Regulating the Pt1-CeO2 interaction via alkali modification for boosting the catalytic performance of single-atom catalysts

被引:7
|
作者
Yang, Peng [1 ,2 ,3 ]
Xu, Juntian [1 ,2 ,3 ]
Tan, Wei [1 ,2 ,3 ]
Liu, Qinglong [1 ,2 ,3 ]
Cai, Yandi [1 ,2 ,3 ]
Xie, Shaohua [4 ]
Hong, Song [5 ]
Gao, Fei [1 ,2 ,3 ]
Liu, Fudong [4 ]
Dong, Lin [1 ,2 ,3 ]
机构
[1] Nanjing Univ, Sch Environm, State Key Lab Pollut Control & Resource Reuse, Nanjing 210023, Peoples R China
[2] Nanjing Univ, Ctr Modern Anal, Jiangsu Key Lab Vehicle Emiss Control, Nanjing 210023, Peoples R China
[3] Nanjing Univ, Sch Chem & Chem Engn, Key Lab Mesoscop Chem MOE, Nanjing 210023, Peoples R China
[4] Univ Cent Florida, Nanosci Technol Ctr NSTC, Catalysis Cluster Renewable Energy & Chem Transfor, Dept Civil Environm & Construction Engn, Orlando, FL 32816 USA
[5] Beijing Univ Chem Technol, Coll Mat Sci & Engn, Beijing 100029, Peoples R China
基金
中国国家自然科学基金;
关键词
TEMPERATURE; SUPPORT; CEO2;
D O I
10.1039/d3cc00387f
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
With the introduction of potassium species, the catalytic oxidation performance over the Pt-1/CeO2 catalyst was significantly enhanced, where potassium ions acted as structural and electronic promoters, and formed Pt-O-K interactions with Pt to directly regulate the coordination environment and electronic state of Pt and the metal-support interaction between Pt and CeO2.
引用
收藏
页码:6219 / 6222
页数:4
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