Simultaneous planar laser-induced fluorescence of nitric oxide and hydroxyl radical with a single dye laser in hydrogen flames

被引:2
|
作者
Chatelain, Karl P. [1 ]
Wang, Guoqing [1 ,3 ]
Guiberti, Thibault F. [1 ,2 ]
机构
[1] King Abdullah Univ Sci & Technol KAUST, Clean Combust Res Ctr CCRC, Thuwal 239556900, Saudi Arabia
[2] KAUST, Div Phys Sci & Engn, Mech Engn Program, Thuwal, Saudi Arabia
[3] KAUST, POB 4700, Thuwal 239556900, Saudi Arabia
关键词
OH-PLIF; NO-PLIF; Spectral coincidence; Sum-frequency generation; Hydrogen combustion; HIGH-PRESSURE FLAMES; OH; DETONATION; STRATEGIES; PLIF; NOX;
D O I
10.1016/j.ijhydene.2023.08.168
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Simultaneous, planar laser-induced fluorescence (PLIF) of nitric oxide (NO) and hydroxyl radical (OH) is evidenced with a single dye laser and two intensified CCD (ICCD) cameras. The technique is demonstrated on three premixed turbulent hydrogen-air flames, at at-mospheric conditions, with several laser excitation wavelengths within the A2S+ -X2P (0,0) and A2S+ -X2P(1,0) vibrational bands of NO and OH, respectively. Via adjustments of the grating angle of the dye laser, the output wavelengths can be optimized so that both LIF signals are obtained simultaneously, or it can be tuned to reach the most common exci-tation wavelengths for OH-PLIF (i.e., near 283 or 284 nm) or NO-PLIF (i.e., 225 and 226 nm) alternatively. The flame visualization results, obtained with the different excitation stra-tegies, are consistent for the three flame conditions and enable to characterize both the reaction zones and the nitric oxide formation. With appropriate selection of the wave-length pair, the technique shows its great potential to enhance the ability of existing lasers to simultaneously visualize and quantify distributions of two key species in reacting flows with only a single laser.(c) 2023 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
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页码:473 / 482
页数:10
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