Removal of levofloxacin and ciprofloxacin from aqueous solutions and an economic evaluation using the electrocoagulation process

被引:35
|
作者
Mohammed, Sabah J. [1 ]
M-Ridha, Mohanad Jasim [1 ]
Abed, Khalid M. [2 ,3 ]
Elgharbawy, Amal A. M. [4 ,5 ]
机构
[1] Univ Baghdad, Coll Engn, Dept Environm Engn, Baghdad, Iraq
[2] Univ Baghdad, Coll Engn, Dept Chem Engn, Baghdad, Iraq
[3] Univ Malaya, Dept Chem Engn, Fac Engn, Kuala Lumpur, Malaysia
[4] Int Islamic Univ Malaysia, Int Inst Halal Res & Training INHART, Kuala Lumpur, Malaysia
[5] Int Islamic Univ Malaysia, Dept Biotechnol Engn, Bioenvironm Engn Res Ctr BERC, Fac Engn, Kuala Lumpur, Malaysia
关键词
Antibiotics; stainless steel electrodes; economic evaluation; kinetic models; isotherm models; wastewater treatment; WASTE-WATER; ADSORPTION; DYE; DECOLORIZATION; OXIDATION; CARBON; TETRACYCLINE; CHROMIUM(VI); PRODUCTS; FLUORIDE;
D O I
10.1080/03067319.2021.1913733
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
For this research, the utilisation of electrocoagulation (EC) toremove theciprofloxacin (CIP) and levofloxacin (LVX) from aqueous solutions was examined. The effective removal efficiencies are 93.47% for CIP and 88.00% for LVX, under optimum conditions. The adsorption isotherm models with suitable mechanisms were applied to determine the elimination of CIP and LVX utilizingtheEC method. Thefindingsshowed the adsorption of CIP and LVX on iron hydroxide flocs followed the Sips isotherm, with correlation coefficient values (R-2) of 0.939 and 0.937. Threekinetic models were reviewed to determine the accurate CIP and LVX elimination methods using the EC method. The results showed that itfittedfor the second-order model, which indicated that the chemical adsorption mechanism controlled the removal of CIP and LVX. The R-2 with CIP is 0.944, and LVX is 0.941. For binary system removal, efficiencies were 93.00, 90.10, and 96.30% for CIP, and 91.80, 96.10, and 92.97% for LVX, at the CIP ratio: LVX of 1:1, 1:4, and 4:1. The electrode consumption (ELC) and electrical energy consumption (EEC) were found at 0.208 g and 3.21 kWh(-3) for a single operation. The operating cost was estimated at 0.613 US$ m(-3).
引用
收藏
页码:3801 / 3819
页数:19
相关论文
共 50 条
  • [31] Removal of arsenic from aqueous solution using electrocoagulation
    Balasubramanian, N.
    Kojima, Toshinori
    Basha, C. Ahmed
    Srinivasakannan, C.
    JOURNAL OF HAZARDOUS MATERIALS, 2009, 167 (1-3) : 966 - 969
  • [32] Evaluation of flurbiprofen removal from aqueous solution by electrosynthesized ferrate(VI) ion and electrocoagulation process
    Barisci, Sibel
    Ulu, Feride
    Sillanpaa, Mika
    Dimoglo, Anatholy
    CHEMICAL ENGINEERING JOURNAL, 2015, 262 : 1218 - 1225
  • [34] Ciprofloxacin removal from aqueous solutions by ozonation with calcium peroxide
    Javid, Neda
    Honarmandrad, Zhila
    Malakootian, Mohammad
    DESALINATION AND WATER TREATMENT, 2020, 174 : 178 - 185
  • [35] Removal of sulfamethoxazole and ciprofloxacin from aqueous solutions by graphene oxide
    Chen, Hao
    Gao, Bin
    Li, Hui
    JOURNAL OF HAZARDOUS MATERIALS, 2015, 282 : 201 - 207
  • [36] Removal of tetracycline and ciprofloxacin from aqueous solutions using magnetic copper ferrite nanoparticles
    Yang, Minge
    He, Jiapan
    He, Junyi
    Cao, Junji
    JOURNAL OF SCIENCE-ADVANCED MATERIALS AND DEVICES, 2024, 9 (02):
  • [37] Contribution of the electrocoagulation method in the removal of fluorine ions from aqueous solutions
    Abbas, Moussa
    DESALINATION AND WATER TREATMENT, 2021, 226 : 177 - 183
  • [38] Modeling of Protein and Phenolic Compound Removal from Aqueous Solutions by Electrocoagulation
    Robic, Goran
    Miranda, Everson Alves
    BIOTECHNOLOGY PROGRESS, 2010, 26 (01) : 186 - 191
  • [39] The effects of alternating current electrocoagulation on dye removal from aqueous solutions
    Eyvaz, Murat
    Kirlaroglu, Mustafa
    Aktas, Tugrul Selami
    Yuksel, Ebubekir
    CHEMICAL ENGINEERING JOURNAL, 2009, 153 (1-3) : 16 - 22
  • [40] Effects of Operational Parameters on the Removal of Tetracycline from Aqueous Solutions by Electrocoagulation
    Moein, Hossein
    Balarak, Davoud
    Meshkinain, Ali
    Chandrika, Kethineni
    Yazdani, Nastaran
    INTERNATIONAL JOURNAL OF PHARMACEUTICAL INVESTIGATION, 2021, 11 (01) : 23 - 26