Geochemical records of human-induced environmental changes in two small remote lakes of Songnen Plain, Northeast China

被引:0
|
作者
Fu, Huan [1 ]
Bao, Kunshan [1 ]
Yu, Jinlei [2 ]
Zhang, Yongdong [1 ]
机构
[1] South China Normal Univ, Sch Geog, Guangzhou 510631, Peoples R China
[2] Chinese Acad Sci, State Key Lab Lake Sci & Environm, Nanjing Inst Geog & Limnol, Nanjing 210008, Peoples R China
关键词
n-Alkanes; Geochemical records; Eutrophication; Nutrients; Catchment disturbance; ORGANIC-MATTER; N-ALKANES; ALIPHATIC-HYDROCARBONS; LIPID BIOMARKERS; SEDIMENTS; CARBON; PETROLEUM; WATER; RECONSTRUCTION; DISTRIBUTIONS;
D O I
10.1007/s11356-023-29733-w
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The abundance and composition of aliphatic hydrocarbon biomarkers were determined in dated sediment cores from Lakes Qijiapao (QJP) and Huoshaoheipao (HSH) in the Songnen Plain, Northeast China, to investigate historical environmental changes in these lakes and identify likely controlling factors. Based on these results, the recent environmental history of the two lakes can be divided into three periods. Before 1950, low P-aq values (avg. 0.23 and 0.27, respectively) and middle-chain n-alkane abundances (normalized to total organic carbon, avg. 14.82 and 16.01 mu g g(-1) TOC, respectively) in both lakes suggested low aquatic productivity and the limited input of submerged macrophyte organic matter (OM). However, the significant increase in the abundance of short-chain n-alkanes in Lake HSH (from 8.34 to 16.68 mu g g(-1) TOC) indicated the emergence of early nutrient enrichment in the lake. From 1950 to 2000, marked increase in the abundance of middle-chain n-alkanes (avg. 21.72 and 22.62 mu g g(-1) TOC in Lakes QJP and HSH, respectively) and P-aq values indicated that both lakes had undergone eutrophication because of the population explosion and agricultural intensification. From 2000 to 2013, the abundance of short- and middle-chain n-alkanes in Lake QJP markedly exceeded those in Lake HSH and indicated a larger eutrophication in Lake QJP, which could be caused by the development of ecotourism in Lake HSH and the concomitant increase in aquaculture in Lake QJP in recent years. The highest abundance of C-30 alpha beta-hopane (similar to 10.24 mu g g(-1) TOC) and the lowest CPIH values in Lake QJP revealed a possible petroleum pollution since 2008. Taken together, lake eutrophication in the Songnen Plain accelerated after 1950 and was influenced primarily by agriculture and aquaculture. This is in contrast to lakes in other regions of China (such as the Yangtze River Basin and Yunnan Province), where urbanization and industrialization have exerted a dominant influence on the lake environment.
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页码:103910 / 103920
页数:11
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