Machine learning for industrial processes: Forecasting amine emissions from a carbon capture plant

被引:13
|
作者
Jablonka, Kevin Maik [1 ]
Charalambous, Charithea [2 ]
Fernandez, Eva Sanchez [3 ]
Wiechers, Georg [4 ]
Monteiro, Juliana [5 ]
Moser, Peter [4 ]
Smit, Berend [1 ]
Garcia, Susana [2 ]
机构
[1] EPFL, Lab Mol Simulat, LSMO, Sion, Switzerland
[2] Heriot Watt Univ, Res Ctr Carbon Solut, Sch Engn & Phys Sci, Edinburgh EH14 4AS, Scotland
[3] Solverlo Ltd, Dunbar EH42 1TL, Scotland
[4] RWE Power, Ernestinenstra 60, D-45141 Essen, Germany
[5] TNO, Leeghwaterstr 44, NL-2628 CA Delft, Netherlands
关键词
POSTCOMBUSTION CO2 CAPTURE; FLEXIBLE OPERATION; PILOT-PLANT; MEA;
D O I
10.1126/sciadv.adc9576
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
One of the main environmental impacts of amine-based carbon capture processes is the emission of the solvent into the atmosphere. To understand how these emissions are affected by the intermittent operation of a power plant, we performed stress tests on a plant operating with a mixture of two amines, 2-amino-2-methyl-1-prop-anol and piperazine (CESAR1). To forecast the emissions and model the impact of interventions, we developed a machine learning model. Our model showed that some interventions have opposite effects on the emissions of the components of the solvent. Thus, mitigation strategies required for capture plants operating on a single component solvent (e.g., monoethanolamine) need to be reconsidered if operated using a mixture of amines. Amine emissions from a solvent-based carbon capture plant are an example of a process that is too complex to be described by conventional process models. We, therefore, expect that our approach can be more generally applied.
引用
收藏
页数:11
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