High-energy-resolution off-resonant spectroscopy with self-seeded x-ray free-electron laser pulses

被引:0
|
作者
Sohn, Jang Hyeob [1 ]
Kang, Gyeongbo [2 ]
Choi, Tae-Kyu [2 ]
Lee, Gyusang [1 ,3 ]
Lee, Changhoo [1 ]
Chun, Sae Hwan [2 ]
Park, Jaeku [2 ]
Shin, Dongbin [1 ,4 ,5 ]
Cho, Byoung-Ick [1 ,3 ]
机构
[1] Gwangju Inst Sci & Technol, Dept Phys & Photon Sci, Gwangju 61005, South Korea
[2] POSTECH, XFEL Div, Pohang Accelerator Lab, Pohang 37673, Gyeongbuk, South Korea
[3] Inst Basic Sci, Ctr Relativist Laser Sci, Gwangju 61005, South Korea
[4] Max Planck Inst Struct & Dynam Matter, D-22761 Hamburg, Germany
[5] Ctr Free Electron Laser Sci, D-22761 Hamburg, Germany
来源
STRUCTURAL DYNAMICS-US | 2024年 / 11卷 / 02期
基金
新加坡国家研究基金会;
关键词
ABSORPTION SPECTROSCOPY; EMISSION-SPECTROSCOPY; SCATTERING; PT/AL2O3;
D O I
10.1063/4.0000243
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
This paper presents the implementation of high-energy-resolution off-resonant spectroscopy (HEROS) measurements using self-seeded x-ray free-electron laser (XFEL) pulses. This study systematically investigated XFEL conditions, including photon energy and accumulated shot numbers, to optimize the measurement efficiency for copper foil samples near the K-edge. The x-ray absorption spectra reconstructed using HEROS were compared with those derived from fluorescence-yield measurements. The HEROS-based spectra exhibited consistent line shapes independent of the sample thickness. The potential application of HEROS to high-temperature copper was also explored. HEROS offers distinct advantages including scan-free measurement of x-ray absorption spectra with reduced core-hole lifetime broadening and self-absorption effects. Using self-seeded XFEL pulses, HEROS facilitates single-shot-based pump-probe measurements to investigate the ultrafast dynamics in various materials and diverse conditions.
引用
收藏
页数:8
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