TiO2/Activated Carbon/2D Selenides Composite Photocatalysts for Industrial Wastewater Treatment

被引:5
|
作者
Ahmad, Shehzad [1 ]
Tahir, Muhammad Suleman [2 ,3 ]
Kamal, Ghulam Mustafa [1 ,4 ]
Zhang, Xu [5 ,6 ,7 ]
Nazir, Saima [4 ,8 ]
Tahir, Muhammad Bilal [9 ]
Jiang, Bin [5 ,6 ,7 ]
Safdar, Muhammad [1 ]
机构
[1] Khwaja Fareed Univ Engn & Informat Technol, Inst Chem, Rahim Yar Khan 64200, Pakistan
[2] Khwaja Fareed Univ Engn & Informat Technol, Inst Chem & Environm Engn, Rahim Yar Khan 64200, Pakistan
[3] Univ Gujrat, Dept Chem Engn, Gujrat 50700, Pakistan
[4] Khwaja Fareed Univ Engn & Informat Technol, Inst Hlth Sci, Rahim Yar Khan 64200, Pakistan
[5] Opt Valley Lab, Wuhan 430074, Peoples R China
[6] Chinese Acad Sci, Wuhan Inst Phys & Math, Innovat Acad Precis Measurement Sci & Technol, Natl Ctr Magnet Resonance Wuhan,Key Lab Magnet Res, Wuhan 430074, Peoples R China
[7] Huazhong Univ Sci & Technol, Wuhan Natl Lab Optoelect, Wuhan 430071, Peoples R China
[8] Univ Gujrat, Nawaz Sharif Med Coll, Gujrat 50700, Pakistan
[9] Khwaja Fareed Univ Engn & Informat Technol, Inst Phys, Rahim Yar Khan 64200, Pakistan
基金
中国国家自然科学基金;
关键词
TiO(2)activated carbon; 2D selenides; photocatalyst; wastewater treatment; GRAPHENE SAND COMPOSITE; TIO2; NANOPARTICLES; OPTICAL-PROPERTIES; DOPED TIO2; DEGRADATION; NANOTECHNOLOGY; MOS2; DYE; OXYTETRACYCLINE; MINERALIZATION;
D O I
10.3390/w15091788
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Even in the 21st century, water contamination has been a big problem and industrial processes are to be blamed for polluted water supplies. The use of sunlight in the process of photocatalysis is an efficientway to purifywastewater. Composites of TiO2/activated carbon/two-dimensional selenides performed better than either of the individual material or binary composites for this application. A straightforward hydrothermal technique was employed in the synthesis of photocatalysts. The synthesized photocatalytic composites were verified with the help of UV-Visible spectroscopy, FTIR, XRD, and SEM. The heterostructures absorbed nearly all of the sun's UV and visible light. These photons are then converted into usable reducing electrons and oxidizing species such as O-center dot(2) and OH center dot to decompose organic pollutants from industrial wastewater. Since there were additional pathways available for charge transfer along with several active edge sites, the composite photocatalysts are proven more active than individual TiO2 and 2D MoSe2 components. With the help of a cascadedriven mechanism of electrons, these channels can transmit more charges than single-component heterojunctions. The results provided a realistic method for developing photocatalyst composites powered by solar light for use in industrial wastewater treatment. Results of degradation of methylene blue suggest that the synthesized composites possess better photocatalytic activity. This enhanced photocatalytic activity is not limited to organic dyes. Other hazardous organic pollutants present in industrial wastewater can be decomposed by using this approach.
引用
收藏
页数:22
相关论文
共 50 条
  • [41] Adsorption properties and photocatalytic activity of TiO2/activated carbon fiber composite
    Shuhua Yao
    Shuangping Song
    Zhongliang Shi
    Russian Journal of Physical Chemistry A, 2014, 88 : 1066 - 1070
  • [42] Fabrication of Carbon Nanotube/TiO2 Composite Photocatalysts and Their Electro-photolysis for Organic Dye
    Zhang, F. J.
    Chen, M. L.
    Oh, W. C.
    ASIAN JOURNAL OF CHEMISTRY, 2009, 21 (09) : 7077 - 7092
  • [43] Lignin-derived carbon and activated carbon nanocomposites with TiO2 as enhanced photocatalysts for organic pollutant degradation
    Montazeri, Reza
    Barbari, Zeinab
    Hosseini-Monfared, Hassan
    Mohammadi, Yasaman
    JOURNAL OF NANOPARTICLE RESEARCH, 2024, 26 (08)
  • [44] Carbon nanotubes/TiO2 nanotubes composite photocatalysts for efficient degradation of methyl orange dye
    Tingshun Jiang
    Lei Zhang
    Meiru Ji
    Qian Wang
    Qian Zhao
    Xiaoqi Fu
    Hengbo Yin
    Particuology, 2013, 11 (06) : 737 - 742
  • [45] Photocatalytic degradation of mixed pollutants in aqueous wastewater using mesoporous 2D/2D TiO2(B)-BiOBr heterojunction
    Liping Han
    Bo Li
    Hao Wen
    Yuxi Guo
    Zhan Lin
    JournalofMaterialsScience&Technology, 2021, 70 (11) : 176 - 184
  • [46] Photocatalytic degradation of mixed pollutants in aqueous wastewater using mesoporous 2D/2D TiO2(B)-BiOBr heterojunction
    Han, Liping
    Li, Bo
    Wen, Hao
    Guo, Yuxi
    Lin, Zhan
    JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY, 2021, 70 : 176 - 184
  • [47] Preparation of GO/TiO2 composite photocatalyst and treatment of synthetic dye wastewater
    Li Dan-dan
    Yao Guang-zheng
    Liang Gui-yan
    Rong Xu-fa
    Xue Ruo-yu
    Fu Zhong-tian
    CAILIAO GONGCHENG-JOURNAL OF MATERIALS ENGINEERING, 2019, 47 (12): : 104 - 110
  • [48] TiO2, TiO2/Ag and TiO2/Au photocatalysts prepared by spray pyrolysis
    Haugen, Astri Bjornetun
    Kumakiri, Izumi
    Simon, Christian
    Einarsrud, Mari-Ann
    JOURNAL OF THE EUROPEAN CERAMIC SOCIETY, 2011, 31 (03) : 291 - 298
  • [49] Adsorption Abilities of Carbon-Modified TiO2 Photocatalysts
    Kusiak, E.
    Janus, M.
    Morawski, A. W.
    PROCEEDINGS OF THE 6TH EUROPEAN MEETING ON SOLAR CHEMISTRY & PHOTOCATALYSIS: ENVIRONMENTAL APPLICATIONS, 2010, : 185 - 186
  • [50] Degradation of phenol in industrial wastewater over the F–Fe/TiO2 photocatalysts under visible light illumination
    Yandong Liu
    Shijian Zhou
    Fu Yang
    Hua Qin
    Yan Kong
    Chinese Journal of Chemical Engineering, 2016, 24 (12) : 1712 - 1718