Research progress on the content and distribution of rare earth elements in rivers and lakes in China

被引:13
|
作者
Traore, Mory [1 ,2 ]
He, Yafei [3 ]
Wang, Yiwen [1 ,2 ]
Gong, Aijun [1 ,2 ]
Qiu, Lina [1 ,2 ]
Bai, Yuzhen [1 ,2 ]
Liu, Yang [1 ,2 ]
Zhang, Min [4 ]
Chen, Yifan [1 ,2 ]
Huang, Xinyu [1 ,2 ]
机构
[1] Univ Sci & Technol Beijing, Sch Chem & Biol Engn, Beijing 100083, Peoples R China
[2] Univ Sci & Technol Beijing, Beijing Key Lab Sci & Applicat Funct Mol & Crystal, Beijing 100083, Peoples R China
[3] Univ Sci & Technol Beijing, Tianjin Coll, Tianjin 301830, Peoples R China
[4] Baotou Water Qual Detect Technol Co Ltd, Baotou 014000, Peoples R China
基金
北京市自然科学基金;
关键词
Rare earth elements (REE); Distribution; Rivers; Lakes; China; SURFACE SEDIMENTS; HEAVY-METALS; GEOCHEMICAL CHARACTERISTICS; SEA IMPLICATIONS; YELLOW-RIVER; TAIHU LAKE; HULUN LAKE; PROVENANCE; ORIGIN; WATER;
D O I
10.1016/j.marpolbul.2023.114916
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This study reviewed the content and distribution of rare earth elements (REE) in rivers and lakes in China based on the online literature. The sequence distribution of REE presented the decreasing trends in the order: of Ce > La > Nd > Pr > Sm > Gb > Dy>Er > Yb > Eu > Lu > Ho > Tb > Tm in rivers water. Pearl River and the Jiulong River constitute a significant sediments REE reservoir with an average value mean of 229.6 mg/kg and 266.86 mg/kg, respectively; both have higher concentrations than the global river average (174.8 mg/kg) and higher than the local soil background (Chinese soil background). The Liaohe River is one of China's most polluted rivers, with REE distribution ranging from 106.61 to 174.71 g/L (average 144.59 g/L in water). The total concentrations of dissolved REE in rivers near REE mining areas in China are higher than in other rivers. Increasing anthro-pogenic inputs to natural systems may permanently alter the natural signatures of REE. The distribution char-acteristics of REE in Chinese lakes (sediments) varied greatly, and the mean enrichment factor (EF) was sorted as follows: Ce > La > Nd > Pr > Sm > Gd > Dy>Er > Yb > Eu > Ho > Tb > Tm > Lu, where Ce was the most abundant followed by La, Nd, and Pr, and these four elements account for 85.39 % of the total concentration of REE. The REE in the sediments obtained from Poyang Lake and Dongting Lake had an average concentration respectively of 254.0 mu g/g and 197.95 mu g/g; both are considerably higher than the average upper continental crust (146.4 mu g/g) and higher than in other lakes in China and around the world. The distribution and accu-mulation of LREE in most lake sediments result from the joint action of human activities and natural processes. It concluded that mining tailings were the primary cause of REE pollution in sediments, and industrial and agri-cultural activities are mainly responsible for water contamination.
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页数:15
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