Resource mining from stainless steel pickling wastewater to produce metal-organic frameworks

被引：40

作者：

Zhao, Xudong ^{[1
]}

Zhang, Chengwei ^{[1
]}

Liu, Baosheng ^{[2
]}

Zhao, Huifang ^{[3
]}

Gao, Xinli ^{[4
]}

Wang, Yuanyang ^{[1
]}

Zhang, Yuezhong ^{[1
]}

Liu, Dahuan ^{[3
]}

Wang, Chong-Chen ^{[5
]}

机构：

[1] Taiyuan Univ Sci & Technol, Coll Chem & Biol Engn, Taiyuan 030024, Peoples R China

[2] Taiyuan Univ Sci & Technol, Coll Mat Sci & Engn, Engn Res Ctr Magnesium Alloy Shanxi Prov, Taiyuan 030024, Peoples R China

[3] Beijing Univ Chem Technol, Coll Chem Engn, State Key Lab Organ Inorgan Composites, Beijing 100029, Peoples R China

[4] Taiyuan Univ Sci & Technol, Instrumental Anal Ctr, Taiyuan 030024, Peoples R China

[5] Beijing Univ Civil Engn & Architecture, Beijing Key Lab Funct Mat Bldg Struct & Environm R, Beijing 100044, Peoples R China

来源：

RESOURCES CONSERVATION AND RECYCLING | 2023年 / 188卷

关键词：

Stainless steel pickling wastewater; Metal -organic framework; Selective crystallization; Resource recycling; AQUEOUS-SOLUTION; EFFECTIVE REMOVAL; ADSORPTION; MIL-100(FE); EQUILIBRIUM; DEGRADATION; CARBOXYLATE; SEPARATION; ZIRCONIUM; MIXTURES;

D O I：

10.1016/j.resconrec.2022.106647

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

Metal-organic frameworks (MOFs) exhibit large potential in many fields while the high cost limits their large-scale use. Herein, stainless steel pickling wastewater was successfully transformed to Fe/Cr-MIL-100, during which Ni2+ was largely purified. As an integration of metal, solvent and acid modifier, the use of the wastewater simplifies the preparation units and reduces the cost of MOFs. Conversion of the pickling wastewater to MOFs is feasible under wide reaction conditions and is not interfered by discharge batch of the wastewater. The obtained MIL-100 s products exhibit excellent porosity, long-term acid/base stability, and large adsorption capacities for methylene blue, moxifloxacin hydrochloride, and zirconium (IV) ion. Thus, our work provides a new insight for effective reuse of industrial wastewater and a feasible method for reducing MOFs cost.

引用

页数：9

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