The Water Quality Index (WQI) is used to monitor the health and usability of a water body. In this study, we aimed to construct time series prediction models using groundwater WQI (GW-WQI) at four sites: IISCO-Asansol, Durgapur Town, Burdwan University, and Burdwan Station. While statistical spatio-temporal analysis has been reported earlier, no time series analysis of the data or predictive modelling has been done. Pre-monsoon and post-monsoon physico-chemical data from 2010 to 2022 were obtained from the West Bengal Pollution Control Board website to calculate the GW-WQI. Prediction modelling was performed using R 4.1.3 software. Best fit forecast models were selected to predict future trends of GW-WQI with 80% of the data. Subsequently, the models were validated using R-squared, root mean square error (RMSE), mean absolute error (MAE), maximum absolute percentage error (MAPE), and Thiel's U for the model using 20% of the data. Our results show that GW-WQI was good in pre-monsoon but unfit for drinking in post-monsoon in IISCO-Asansol, Durgapur Town, Burdwan University, and Burdwan Station. Arsenic, fluoride, and mercury were the major contaminants resulting in poor GW-WQI. Seasonal ARIMA was the best model for Burdwan University and IISCO-Asansol, ETS for Durgapur Station, and BaggedARIMA for Burdwan Station. The forecast model for Durgapur and Burdwan Station predicted a sharp increase until 2027 but was fluctuating for IISCO-Asansol and Burdwan University. Thus, GW-WQI is a major problem in the industrial belt of West Bengal that is likely to remain high or worsen in the future.