high polarization sensitivity;
photogalvanic effects;
quantum transport simulations;
TOTAL-ENERGY CALCULATIONS;
D O I:
10.1002/pssa.202200686
中图分类号:
T [工业技术];
学科分类号:
08 ;
摘要:
The photogalvanic effect (PGE) generated under linearly polarized light irradiation has remarkable applications in 2D nanodevices. The PGE of 2D WS2/Mo2CF2 van der Waals (vdW) heterostructure can generate photocurrent and high sensitivity to polarized light. However, the PGE has less photogenerated current. On this basis, the photocurrent transport mechanism of PGE under low bias voltage is investigated. The results show that the photocurrent of the photon energy has cos 2 theta , sin 2 theta and sin2 theta dependence on the polarization angle theta under the considered external bias voltage. Under a bias voltage of 1.0 V, the maximum photocurrent of 3.7 eV photon energy in the zigzag direction can reach 4.61. Under a bias voltage of 1 V, the maximum photocurrent of 1.8 eV photon energy in the armchair direction can reach 6.71. The maximum photocurrents are in the order of 10(-1) for both zigzag and armchair directions with 0 V bias. Furthermore, 2D WS2/Mo2CF2 vdW heterostructure has a stable and high extinction ratio. These results show that 2D WS2/Mo2CF2 vdW heterostructure is a potential candidate material for future optoelectronics in the visible light region.
机构:
CNR, Ist Nazl Ott, Via Moruzzi 1, I-56124 Pisa, ItalyCNR, Ist Nazl Ott, Via Moruzzi 1, I-56124 Pisa, Italy
Dinelli, Franco
Fabbri, Filippo
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机构:
Scuola Normale Super Pisa, NEST, Piazza San Silvestro 12, I-56127 Pisa, Italy
CNR, Ist Nanosci, NEST, Piazza San Silvestro 12, I-56127 Pisa, Italy
Ist Italiano Tecnol, CNI NEST, Piazza San Silvestro 12, I-56127 Pisa, ItalyCNR, Ist Nazl Ott, Via Moruzzi 1, I-56124 Pisa, Italy
Fabbri, Filippo
Forti, Stiven
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机构:
Ist Italiano Tecnol, CNI NEST, Piazza San Silvestro 12, I-56127 Pisa, ItalyCNR, Ist Nazl Ott, Via Moruzzi 1, I-56124 Pisa, Italy
Forti, Stiven
Coletti, Camilla
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机构:
Ist Italiano Tecnol, CNI NEST, Piazza San Silvestro 12, I-56127 Pisa, Italy
Ist Italiano Tecnol, Graphene Labs, Via Morego 30, I-16163 Genoa, ItalyCNR, Ist Nazl Ott, Via Moruzzi 1, I-56124 Pisa, Italy
Coletti, Camilla
Kolosov, Oleg, V
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机构:
Univ Lancaster, Dept Phys, Lancaster LA1 4YB, EnglandCNR, Ist Nazl Ott, Via Moruzzi 1, I-56124 Pisa, Italy
Kolosov, Oleg, V
Pingue, Pasqualantonio
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机构:
Scuola Normale Super Pisa, NEST, Piazza San Silvestro 12, I-56127 Pisa, ItalyCNR, Ist Nazl Ott, Via Moruzzi 1, I-56124 Pisa, Italy