Role of H-beta zeolite on photocatalytic pollutant degradation and H2 production enhancement of g-C3N4/H-Beta composite

被引:7
|
作者
Yang, Xiaohang [1 ]
Qiao, Jianguo [2 ]
Deng, Jiayuan [2 ]
Jia, Ruokun [2 ]
Wang, Qiyao [1 ]
机构
[1] Jilin Med Univ, Coll Biomed Engn, Jilin 132013, Peoples R China
[2] Northeast Elect Power Univ, Coll Chem Engn, Jilin 132012, Peoples R China
来源
关键词
H-Beta zeolite; Photocatalysis; Pollutant degradation; H2; evolution; HYDROGEN EVOLUTION; H-2; EVOLUTION; G-C3N4; PERFORMANCE; IRRADIATION; ADSORPTION; OXIDATION; UV;
D O I
10.1016/j.jece.2023.110828
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Limited by low surface area and insufficient photoelectric conversion efficiency, bulk g-C3N4 showed unsatisfactory photocatalytic pollutant degradation and H2 evolution performance. Herein, hydrophilic and porous HBeta zeolite was employed to prepare g-C3N4/H-Beta composite via facile in-situ polymerization method. The role of H-Beta zeolite manifested in increased surface area, improved hydrophilicity and facilitated separation and transportation of photoexcited charge carriers. Hence, the obtained g-C3N4/H-Beta photocatalyst with an optimal content of H-Beta zeolite showed highest photocatalytic pollutant degradation efficiency and H2 generation rate, which were 7.31- and 6.32-fold greater than that of bulk g-C3N4.
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收藏
页数:10
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