The double-sided carbonization of poplar with different sections forms a three-layer structure inspired by tree water transpiration. A photothermal evaporation comparison experiment was conducted to simulate the influence of solar radiation intensity (1 kW center dot m(-2)) on uncarbonized and single- and double-sided carbonized poplar specimens. The tissue structure, chemical functional group changes, and profile density of the specimens were analyzed using scanning electron microscopy, Fourier transform infrared spectrometry, and X-ray profile density testing, respectively. The results showed that the tissue structure of the specimen changed after treatment, and the relationship of water evaporation was shown as follows: cross-section (C) > Radial section (R) > Tangential section (T), and Double-sided carbonized poplar (DCP) > Single-sided carbonized poplar (SCP) > Non-carbonized poplar (NCP). Of these, the maximum photothermal evaporation was from the cross-section of the double-sided carbonized poplar (NCPC) with a value of 1.32 kg center dot m(-2)center dot h(-1), which was 21.97% higher than single-sided carbonized poplar (SCPC) and 37.88% higher than non-carbonized poplar (NCPC). Based on the results, double-sided carbonization three-layer structure treatment can improve the evaporation force of the poplar interface, thereby improving the moisture migration ability of wood, and can be applied to solar interface absorber materials.