Conductometric Cr2O3/TiO2/Ti3C2Tx Gas Sensor for Detecting Triethylamine at Room Temperature

被引:27
|
作者
Yao, Yu [1 ,2 ]
Wang, Zifeng [1 ]
Han, Yutong [1 ]
Xie, Lili [2 ]
Zhao, Xueling [2 ]
Shahrokhian, Saeed [3 ]
Barsan, Nicolae [4 ,5 ]
Zhu, Zhigang [1 ]
机构
[1] Univ Shanghai Sci & Technol, Sch Hlth Sci & Engn, Shanghai 200093, Peoples R China
[2] Shanghai Polytech Univ, Sch Energy & Mat, Shanghai 201209, Peoples R China
[3] Sharif Univ Technol SUT, Dept Chem, Tehran, Iran
[4] Univ Tubingen, Inst Phys & Theoret Chem IPTC, Morgenstelle 15, D-72076 Tubingen, Germany
[5] Univ Tubingen, Ctr Light Matter Interact Sensors & Analyt LISA, Morgenstelle 15, D-72076 Tubingen, Germany
基金
中国国家自然科学基金;
关键词
Gas sensor; MXene; Stabilization; Metal oxides; Triethylamine; Environmental detection;
D O I
10.1016/j.snb.2023.133412
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
MXene-based gas-sensitive nanocomposites are an area of high interest in developing high-performance gas sensors that operate at room temperature. Combining MXene with different nano-sized metal oxides is a strategy to improve sensing performance, but poor chemical stability, especially in humid environments, is the biggest obstacle to practical applications. Recently we demonstrated a method to prepare a ternary heterostructure gas sensor by decorating a stable TiO2/Ti3C2Tx composite with MoO3 which also provided selectivity. Here, we develop the proposed concept by synthesizing a Cr2O3/TiO2/Ti3C2Tx gas-sensitive material that shows a unique rapid and selective response to Triethylamine. In addition, the sensor offers excellent chemical stability and can maintain its morphology and gas sensing performance even after ageing at 500 degrees C for two months. This work demonstrates the validity of the proposed approach for an additional metal oxide and yields a sensor that exhibits potential for excellent practical application in harsh environment.
引用
收藏
页数:8
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