Parametric study on reaction characteristics of methane/air mixture in microchannels

被引:1
|
作者
Wang, Yefeng [1 ,2 ]
Wang, Shuai [3 ]
Ye, Hengdi [1 ]
Zhou, Haoyu [1 ]
Zhu, Rong [2 ]
Wei, Jinchao [1 ]
Peng, Yaqi [3 ]
Yang, Weijuan [3 ]
机构
[1] Zhongye Changtian Int Engn Co Ltd, Natl Engn Res Ctr Sintering & Pelletizing Equipmen, Changsha 410205, Peoples R China
[2] Univ Sci & Technol Beijing, Sch Met & Ecol Engn, Beijing 100083, Peoples R China
[3] Zhejiang Univ, State Key Lab Clean Energy Utilizat, Hangzhou 310027, Peoples R China
关键词
Catalytic combustion; Methane; Heterogeneous reaction; Homogeneous reaction; Operating parameters; HETEROGENEOUS REACTION CHARACTERISTICS; HETERO-/HOMOGENEOUS COMBUSTION; ASSISTED CATALYTIC COMBUSTION; HOMOGENEOUS COMBUSTION; WALL SURFACE; AIR MIXTURES; GAS-PHASE; FLAME; EXTINCTION; SIMULATION;
D O I
10.1016/j.ces.2023.119500
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Micro-combustion is a promising technology for addressing global energy consumption challenges; however, its practical implementation is hindered by a limited understanding of the underlying reaction characteristics. To address this, a comprehensive numerical investigation was conducted using a well-established two-dimensional (2D) steady model to examine the influence of key operating parameters (e.g., inlet velocity, equivalence ratio, and inlet temperature) on catalytic methane/air combustion in micro-channels. The results show that the het-erogeneous reaction exhibits limited sensitivity to changes in inlet velocity, whereas the homogeneous reaction shows substantial enhancement with increasing inlet temperature. With the increment of inlet velocity, the peak value of stage III-heterogeneous ignition (conversion of CO to CO2 and H-2 to H2O) decreases and levels off once u(in) >= 0.50 m/s. Simultaneously, the minimum value of S (the ratio of heat released by the heterogeneous reaction to that of the total reaction) decreases as well. As the equivalence ratio is increased, the combustion zone shifts towards the upstream direction. The value of S initially increases and then decreases, reaching a maximum of 17.61 % at Phi = 0.95. Raising the inlet temperature results in the upstream movement of the flame, accompanied by reduced combustion heat release, lower combustion temperature, and diminished intensity of homogeneous combustion. The influence of the heterogeneous reaction on combustion is more pronounced under operating conditions with lower inlet velocities, an equivalence ratio approaching 0.95, and higher inlet temperature. Additionally, under the condition of higher inlet velocities, an equivalence ratio close to 1.0, and elevated inlet temperature, the heterogeneous reaction aids in igniting the homogeneous reaction more effectively.
引用
收藏
页数:14
相关论文
共 50 条
  • [31] Direct observations of reaction zone structure in shock-induced ignition of methane air mixture
    Wang GaoFeng
    Ma ChengBiao
    Wang BaoYuan
    Lin QiZhao
    CHINESE SCIENCE BULLETIN, 2009, 54 (13): : 2247 - 2255
  • [32] Numerical investigation on dynamic flow characteristics of methane condensation in microchannels
    Sun, Yuwei
    Zhao, Cong
    Wang, Haocheng
    Qiu, Yinan
    Gong, Maoqiong
    Zhao, Yanxing
    INTERNATIONAL JOURNAL OF REFRIGERATION, 2024, 167 : 185 - 200
  • [33] STUDY ON METHANE-AIR MIXTURE IGNITION IN THE SHOCK TUBE: STUDIES ON METHANE-AIR MIXTURE IGNITION CAUSED BY SHOCK WAVES (1ST REPORT).
    Shibuya, Takashi
    Isobe, Toshiro
    1984, (100):
  • [34] Study of flame development in 12% methane-air mixture ignited by laser
    Salamu, G.
    Sandu, O.
    Voicu, F.
    Dejanu, M.
    Popa, D.
    Parlac, S.
    Ticos, C.
    Pavel, N.
    Dascalu, T.
    OPTOELECTRONICS AND ADVANCED MATERIALS-RAPID COMMUNICATIONS, 2011, 5 (11): : 1166 - 1169
  • [35] The effect of ethane on the chain reaction characteristics of methane-air mixtures explosions
    Li, Xiangchun
    Liu, Yi
    Yang, Chunli
    Chen, Zhifeng
    Yang, Wenlong
    JOURNAL OF LOSS PREVENTION IN THE PROCESS INDUSTRIES, 2024, 91
  • [36] Transition to oscillatory instability of lean methane-air flames in microchannels
    Yakovlev, Igor
    Fursenko, Roman
    Astakhov, Daniil
    Zambalov, Sergey
    Maznoy, Anatoly
    COMBUSTION AND FLAME, 2024, 267
  • [37] Heat transfer characteristics of flame jet impingement with methane air reaction environment
    Agarwal, A.
    Letsatsi, M. T.
    MATERIALS TODAY-PROCEEDINGS, 2021, 39 : 789 - 795
  • [38] Combustion characteristics of homogeneous charged methane-air mixture in a constant volume combustion chamber
    Choi, SH
    Cho, SW
    Jeong, DS
    Jeon, CH
    Chang, YJ
    INTERNATIONAL JOURNAL OF AUTOMOTIVE TECHNOLOGY, 2005, 6 (04) : 323 - 332
  • [40] Effects of N2/CO2 on explosion characteristics of methane and air mixture
    Wang, Z. R.
    Ni, L.
    Liu, X.
    Jiang, J. C.
    Wang, R.
    JOURNAL OF LOSS PREVENTION IN THE PROCESS INDUSTRIES, 2014, 31 : 10 - 15