Optical and thermoluminescence properties of Lu2Si2O7:Pr single crystal

被引:0
|
作者
冯鹤 [1 ]
任国浩 [2 ]
吴云涛 [2 ]
徐军 [2 ]
杨秋红 [1 ]
谢建军 [1 ]
周明奇 [3 ]
陈晨龙 [3 ]
机构
[1] School of Materials Science and Engineering, Shanghai University
[2] Shanghai Institute of Ceramics, Chinese Academy of Science
[3] Department of Materials & Opto-electronic Science, National Sun Yat-Sen University
基金
上海市自然科学基金; 中国国家自然科学基金;
关键词
Pr3+ doped lutetium pyrosilicate; single crystal; scintillation; optical properties; thermally stimulated luminescence; rare earths;
D O I
暂无
中图分类号
O614.33 [镧系元素(稀土元素)];
学科分类号
070301 ; 081704 ;
摘要
Single crystal of Lu2Si2O7:Pr was grown by Czochralski method. Transmittance, photoluminescence excitation (PLE) and photo-luminescence (PL) spectra, X-ray excited luminescence (XEL) and fluorescence decay time spectra of the sample were measured and discussed to investigate its optical characteristics. The crystal structure of the as grown Lu2Si2O7:Pr was confirmed to be C2/m. There was a broad absorption peaking at 245 nm in the region from 200-260 nm. The PL spectrum was dominated by fast 3PJ→3HJ band peaking at 524 nm. The XEL spectrum was dominated by the fast 5d14f1→4f2 emission peaking at 265 nm. The 2D (temperature-intensity) and 3D (temperature-wavelength-intensity) thermally stimulated luminescence (TSL) spectra were measured. The Pr3+ ion was found to be the recombination center during the TSL process. Three obvious traps were detected in LPS:Pr single crystal with energy depth at 1.06, 0.78 and 0.67 eV.
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页码:775 / 779
页数:5
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