Let n be a natural number, and let A be an indecomposable cellular algebra such that the spectrum of its Cartan matrix C is of the form {n, 1, …., 1}. In general, not every natural number could be the number of non-isomorphic simple modules over such a cellular algebra. Thus, two natural questions arise: (1) which numbers could be the number of non-isomorphic simple modules over such a cellular algebra A ? (2) Given such a number, is there a cellular algebra such that its Cartan matrix has the desired property ? In this paper, we shall completely answer the first question, and give a partial answer to the second question by constructing cellular algebras with the pre-described Cartan matrix.