Exploring superconductivity under strong coupling with the vacuum electromagnetic field

被引:0
|
作者
Thomas, A. [1 ,2 ,3 ,6 ]
Devaux, E. [1 ,2 ,3 ]
Nagarajan, K. [1 ,2 ,3 ,7 ]
Chervy, T. [1 ,2 ,3 ,8 ]
Seidel, M. [1 ,2 ,3 ,9 ]
Rogez, G. [1 ,4 ]
Robert, J. [1 ,4 ]
Drillon, M. [1 ,4 ]
Ruan, T. T. [5 ]
Schlittenhardt, S. [5 ]
Ruben, M. [1 ,2 ,3 ,5 ]
Hagenmueller, D. [1 ,2 ,3 ]
Schutz, S. [1 ,2 ,3 ]
Schachenmayer, J. [1 ,2 ,3 ]
Genet, C. [1 ,2 ,3 ]
Pupillo, G. [1 ,2 ,3 ]
Ebbesen, T. W. [1 ,2 ,3 ]
机构
[1] Univ Strasbourg, F-67000 Strasbourg, France
[2] CNRS, ISIS, F-67000 Strasbourg, France
[3] CESQ, F-67000 Strasbourg, France
[4] CNRS, IPCMS, F-67000 Strasbourg, France
[5] Karlsruhe Inst Technol, Inst Nanotechnol, D-76344 Eggenstein Leopoldshafen, Germany
[6] IISc, Dept Inorgan & Phys Chem, Bengaluru, India
[7] TIFR, Dept Chem Sci, Mumbai, India
[8] PHI Labs, NTT Res, Sunnyvale, CA 94085 USA
[9] DESY, Hamburg, Germany
来源
JOURNAL OF CHEMICAL PHYSICS | 2025年 / 162卷 / 13期
关键词
LIGHT-INDUCED SUPERCONDUCTIVITY; STATE CHEMICAL-REACTIVITY; TRANSITION-TEMPERATURE; CAVITY; K3C60;
D O I
10.1063/5.0231202
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Strong light-matter interactions have generated considerable interest as a means to manipulate material properties. Here, we explore this possibility with the molecular superconductor Rb3C60 under vibrational strong coupling (VSC) to surface plasmon polaritons. By placing the superconductor-surface plasmon system in a SQUID magnetometer, we find that the superconducting transition temperature (T-c) increases from 30 to 45 K at normal pressures under VSC, displaying a well-defined Meissner effect. A simple theoretical framework is provided to understand these results based on an enhancement of the electron-phonon coupling. This proof-of-principle study opens a new tool box to not only modify superconducting materials but also to understand the mechanistic details of different superconductors.
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页数:7
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