Au supported on γ-AlOOH and γ-Al2O3 for low temperature oxidation of CO and aromatic alcohols

被引:0
|
作者
Shi, Zongbo [1 ]
Zhang, Qing [1 ]
Yang, Guangpeng [1 ]
Liu, Liang [1 ]
Wang, Gang [2 ]
Ekananda, Rizki [3 ]
Gamar, Ismal [3 ]
Wang, Ruilin [2 ]
Zhuo, Runsheng [1 ]
机构
[1] Rezel Catalysts Corp, Shanghai 201313, Peoples R China
[2] Sichuan Univ, Coll Mat Sci & Engn, Chengdu 610065, Peoples R China
[3] PT Pertamina Persero, E Jakarta 13920, Indonesia
关键词
GOLD NANOPARTICLES; AEROBIC OXIDATION; CATALYSTS; BOEHMITE; PERFORMANCE; ALUMINA; OXIDE; TIO2;
D O I
10.1039/d5ra00527b
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
0.5%Au supported on gamma-AlOOH and gamma-Al2O3 was used for low temperature oxidation of CO and aromatic alcohols. Various characterization techniques, including X-ray diffraction, N2 adsorption, FT-IR spectroscopy, XPS, TEM, CO2-TPD and solid-state MAS NMR, were employed to characterize these catalysts. The Au/gamma-AlOOH sample has abundant hydroxyl groups and basic sites on its surface, exhibiting strong adsorption for aromatic alcohols, and outstanding activity for low-temperature oxidation of aromatic alcohols. The Au/gamma-Al2O3 sample shows sufficient Au+ sites leading to high performance for low-temperature CO oxidation.
引用
收藏
页码:7563 / 7570
页数:8
相关论文
共 50 条
  • [31] Oxidation of CO and Propane on Pt-Au/Al2O3 Catalysts
    Ruszel, M.
    Grzybowska-Swierkosz, B.
    Karpinski, Z.
    Juszczyk, W.
    POLISH JOURNAL OF CHEMISTRY, 2008, 82 (10) : 1991 - 1997
  • [32] On the mechanism of selective CO oxidation on nanosized Au/γ-Al2O3 catalysts
    Gavril, D.
    Georgaka, A.
    Loukopoulos, V.
    Karaiskakis, G.
    Nieuwenhuys, B. E.
    GOLD BULLETIN, 2006, 39 (04) : 192 - 199
  • [33] Oxidation of CO by au on highly active Al2O3 support.
    Lindquist, DA
    Rimmer, RD
    Perry, DA
    Shekhawat, R
    Sharma, R
    Davis, BJ
    Mazumder, MK
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2004, 227 : U1564 - U1564
  • [34] The active phase of Au-Pd/Al2O3 for CO oxidation
    Suo, Zhanghuai
    Ma, Chunyan
    Jin, Mingshan
    He, Tao
    An, Lidun
    CATALYSIS COMMUNICATIONS, 2008, 9 (13) : 2187 - 2190
  • [35] CO oxidation over Au/Al2O3 catalysts modified by MgO
    Szabó, EG
    Hegedus, M
    Szegedi, A
    Sajó, I
    Margitfalvi, JL
    REACTION KINETICS AND CATALYSIS LETTERS, 2005, 86 (02): : 339 - 345
  • [36] On the mechanism of selective CO oxidation on nanosized Auγ-Al2O3 catalysts
    D Gavrila
    A Georgakab
    V Loukopoulosb
    G Karaiskakisb
    B E Nieuwenhuysa
    Gold Bulletin, 2006, 39 : 192 - 199
  • [37] Synergism Between Pt/Al2O3 and Au/TiO2 in the Low Temperature Oxidation of Propene
    D.H. Kim
    M.C. Kung
    A. Kozlova
    S.D. Yuan
    H.H. Kung
    Catalysis Letters, 2004, 98 : 11 - 15
  • [38] Synergism between Pt/Al2O3 and Au/TiO2 in the low temperature oxidation of propene
    Kim, DH
    Kung, MC
    Kozlova, A
    Yuan, SD
    Kung, HH
    CATALYSIS LETTERS, 2004, 98 (01) : 11 - 15
  • [39] An excellent Au/meso-γ-Al2O3 catalyst for the aerobic selective oxidation of alcohols
    Zhao, Guofeng
    Ling, Min
    Hu, Huanyun
    Deng, Miaomiao
    Xue, Qingsong
    Lu, Yong
    GREEN CHEMISTRY, 2011, 13 (11) : 3088 - 3092
  • [40] Supported Au catalysts for low temperature CO oxidation
    Kung, HH
    Kung, MC
    Costello, CK
    JOURNAL OF CATALYSIS, 2003, 216 (1-2) : 425 - 432