Transition metal nickel nanoparticle-decorated g-C3N4 photocatalyst for improving tetracycline hydrochloride degradation

被引:0
|
作者
Nguyen, Oanh T. K. [1 ]
Nguyen, Vinh Huu [1 ]
Nong, Linh Xuan [1 ]
Doan, Que-Minh T. [1 ]
Hoang, Lan-Anh T. [2 ]
Nam, Kwang Hee [3 ]
Lee, Taeyoon [2 ]
Nguyen, Trinh Duy [1 ]
机构
[1] Nguyen Tat Thanh Univ, Inst Appl Technol & Sustainable Dev, Ho Chi Minh City, Vietnam
[2] Pukyong Natl Univ, Coll Environm & Marine, Dept Environm Engn, 45 Yongso Ro, Busan 48513, South Korea
[3] Pukyong Natl Univ, Ind Univ Cooperat Fdn, 45 Yongso Ro, Busan 48513, South Korea
关键词
Photocatalyst; Photodegradation; Tetracycline; Graphite carbonitrile; GRAPHITIC CARBON NITRIDE; DOPED G-C3N4; BAND-STRUCTURE; SOLAR; HETEROJUNCTION; REDUCTION; NI; PHOTODEGRADATION; CONSTRUCTION; ENVIRONMENT;
D O I
10.1016/j.jphotochem.2024.116042
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Metallic nickel nanoparticles (Ni0 NPs)-supported g-C3N4 have been developed using a solvothermal technique in N,N-dimethylformamide solvent. A uniformly dispersion of Ni0 NPs anchored on a g-C3N4 photocatalyst can improve the photocatalytic efficiency. The optimized Ni/g-C3N4 catalyst demonstrated a high photodegradation rate of TCH at 6.0 x 10-3 min-1 under LED light irradiation, which was approximately three times greater than that of the bare g-C3N4 catalyst. This superior performance originates from the capable separation of electron- hole pairs, facilitated by the strong interaction between Ni0 NPs and the host g-C3N4, as supported by optical and electrochemical property analysis. Our work provides a facile manner for the effective degradation of pollutants using heterojunction photocatalysts.
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页数:9
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