A magneto-thermoelectric with a high figure of merit in topological insulator Bi88Sb12

被引:2
|
作者
Pan, Yu [1 ,2 ,3 ]
He, Bin [1 ]
Feng, Xiaolong [1 ]
Li, Fan [4 ,5 ]
Chen, Dong [1 ]
Burkhardt, Ulrich [1 ]
Felser, Claudia [1 ]
机构
[1] Max Planck Inst Chem Phys Solids, Dresden, Germany
[2] Chongqing Univ, Coll Mat Sci & Engn, Chongqing, Peoples R China
[3] Chongqing Univ, Ctr Quantum Mat & Devices, Chongqing, Peoples R China
[4] Max Planck Inst Microstruct Phys, NISE Dept, Halle, Germany
[5] Chongqing Univ, Coll Phys, Chongqing, Peoples R China
基金
中国国家自然科学基金;
关键词
PERFORMANCE; BI;
D O I
10.1038/s41563-024-02059-9
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
High thermoelectric performance is generally achieved by synergistically optimizing two or even three of the contradictorily coupled thermoelectric parameters. Here we demonstrate magneto-thermoelectric correlation as a strategy to achieve simultaneous gain in an enhanced Seebeck coefficient and reduced thermal conductivity in topological materials. We report a large magneto-Seebeck effect and high magneto-thermoelectric figure of merit of 1.7 +/- 0.2 at 180 K and 0.7 T in a single-crystalline Bi88Sb12 topological insulator. This result fills a gap of a high performance below 300 K and is promising for low-temperature thermoelectric applications. The large magneto-Seebeck response is attributed to the ultrahigh mobility and the Dirac band dispersion. The application of a low magnetic field to achieve a high thermoelectric performance can be extended to topological materials with similar features that are rapidly emerging because it synergistically optimizes the thermoelectric parameters.
引用
收藏
页码:76 / 82
页数:9
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