High-performance single-component white light-emitting diodes based on donor-acceptor integrated carbon nitride

被引:0
|
作者
Ning Wu [1 ]
Fangxu Dai [1 ,2 ]
Kunpeng Wang [1 ]
Yunhu Wang [1 ]
Xinyi Wang [1 ]
Kai Zhang [1 ]
Mingming Zhang [1 ,3 ]
Kang Liu [1 ]
Jixiang Xu [1 ]
Lei Wang [1 ]
Jun Xing [1 ]
机构
[1] Key Laboratory of Eco-chemical Engineering,Ministry of Education,College of Chemistry and Molecular Engineering,Qingdao University of Science & Technology
[2] School of Pharmacy,Jining Medical University
[3] College of Sino-German Science and Technology,Qingdao University of Science &
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中图分类号
TN312.8 []; TQ127.16 [];
学科分类号
0803 ;
摘要
White light-emitting diodes(WLEDs) as energy-saving light sources are widely used to alleviate the rising electric consumption.Most commercial WLEDs are blue/yellow-mixed emitting devices,which have some disadvantages,such as physiological damages of rich blue light,complex device structure and color aging.It is essential to develop single-component WLEDs with quasi-solar spectrum to overcome these problems.Here we demonstrate a high-performance single-component WLED based on donor-acceptor integrated carbon nitride(DACN) material.The donor-acceptor simultaneously increases the photoluminescence efficiency and the carrier mobility of graphitic carbon nitride(g-CN),hence,the DACN-based WLED reaches a milestone in maximum luminance of 2,045 cdm-2 and maximum external quantum efficiency of 2.2%,which are one order of magnitude higher than pristine g-CN-based LED.Furthermore,the DACN-based WLED emits broadband white light with color coordinates of(0.34,0.44) and a color temperature of 5,163 K.Our works open a way to boost optoelectronic properties of g-CN materials and show their promising application in single-component WLEDs.
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页码:1136 / 1143
页数:8
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