High-temperature dehydrogenation of Brønsted acid sites in zeolites

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Nash, Michael J.
Shough, Anne Marie
Fickel, Dustin W.
Doren, Douglas J.
Lobo, Raul F.
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We present evidence for the dehydrogenation of zeolite Brønsted acid sites at temperatures above 500 °C forming hydrogen gas and a [AlO4]0 site that could participate in one-electron oxidations or react further to form extraframework aluminum. Copyright © 2008 American Chemical Society;
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页码:2460 / 2462
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