Comprehensive analysis and risk assessment of fine road dust in Abbottabad city (Pakistan) with heavy traffic for potentially toxic elements

被引:2
|
作者
Jadoon, Waqar Azeem [1 ]
Khan, Yousaf Ali [2 ]
Varol, Memet [3 ]
Onjia, Antonije [4 ]
Mohany, Mohamed [5 ]
机构
[1] Hazara Univ Mansehra, Dept Earth & Environm Sci, Mansehra 21130, Pakistan
[2] Hazara Univ Mansehra, Dept Math & Stat, Mansehra 21130, Pakistan
[3] Malatya Turgut Ozal Univ, Agr Fac, Aquaculture Dept, Malatya, Turkiye
[4] Univ Belgrade, Fac Technol & Met, Karnegijeva 4, Belgrade 11120, Serbia
[5] King Saud Univ, Coll Pharm, Dept Pharmacol & Toxicol, POB 55760, Riyadh 11451, Saudi Arabia
关键词
Fine road dust; PTEs; Traffic pollution; APCS-MLR; Health risk assessment; Abbottabad; Pakistan; METAL CONTAMINATION; TRACE-ELEMENTS; HEALTH-HAZARDS; SOILS; APPORTIONMENT; SIALKOT;
D O I
10.1016/j.jhazmat.2024.136788
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Human activities have far-reaching impact on natural ecosystems, causing increasing disturbances and disruptions to the delicate balance of the environment. Poor land use planning, urbanization, infrastructure development, and unplanned tourism exacerbate contamination and degradation in tourist destinations, yet the pollution of potentially toxic elements (PTEs) in these environments remains inadequately explored. To address this issue, we investigated the concentrations of acid-digested PTEs in road dust in Abbottabad city (Pakistan) with heavy traffic. The current study also evaluated PTE associated pollution, ecological and health risks, and potential sources of these elements. The average concentrations (in mg kg-1) of PTEs in road dust were highest for Fe (15540), followed by Mn (304), Zn (139), Cu (50.0), Pb (21.5), Cr (13.0), Ni (10.3), Co (6.66), and Cd (0.236). The levels of Co, Cr, Mn, Ni, and Fe were below the upper continental crust (UCC) averages, while Cd, Cu, Pb, and Zn exceeded them. Spatially, Cd, Cu, Pb, and Zn were found at higher levels near traffic hotspots, bus stands and automobile workshops. Road dust in Abbottabad exhibited unpolluted to moderate pollution levels (geo accumulation index), with Cd, Cu, Zn, and Pb at 23 % of the sites. The enrichment factor results indicated a significant anthropogenic influence, with Cd being significantly enriched and Zn, Cu, and Pb moderately enriched. The contamination factor results revealed moderate contamination by (Cd: 2.62, Zn: 2.08, Cu: 1.79, Pb: 1.27). Single metal risk index showed that 61 % of the sites posed considerable to very high ecological risks due to Cd, which was highlighted as a significant concern. The absolute principal component scores-multiple linear regression model identified three factors contributing to PTE pollution: lithogenic (Co, Fe, Mn, Ni), traffic-related (Cd, Cu, Pb, Zn), and mixed sources (Cr), with contributions of 52.8 %, 35.8 %, and 11.4 %, respectively. The PTE hazard quotient and total hazard index values for children and adults were below the safe risk level of 1, indicating no non-carcinogenic health risks. The cumulative carcinogenic risk values to the residents were also within acceptable limits. However, children's susceptibility to non-carcinogenic risks is higher due to their behavior and lower body weight. This study highlights the accumulation of PTEs in Abbottabad's environment, which poses challenges to long-term sustainability, particularly amid unplanned tourism. Therefore, urgent measures are necessary to mitigate PTE pollution and preserve tourist spots and public health.
引用
收藏
页数:13
相关论文
共 50 条
  • [41] Pollution status and human health risk assessment of potentially toxic elements and polycyclic aromatic hydrocarbons in urban street dust of Tyumen city, Russia
    Konstantinova, Elizaveta
    Minkina, Tatiana
    Konstantinov, Alexandr
    Sushkova, Svetlana
    Antonenko, Elena
    Kurasova, Alina
    Loiko, Sergey
    ENVIRONMENTAL GEOCHEMISTRY AND HEALTH, 2022, 44 (02) : 409 - 432
  • [42] Pollution of a Black Sea coastal city: potentially toxic elements in urban soils, road dust, and their PM10 fractions
    Bezberdaya, Liliya
    Chernitsova, Olga
    Lychagin, Mikhail
    Aseeva, Elena
    Tkachenko, Anna
    Kasimov, Nikolay
    JOURNAL OF SOILS AND SEDIMENTS, 2024, 24 (10) : 3485 - 3506
  • [43] A comparative study of health risk of potentially toxic metals in urban and suburban road dust in the most populated city of China
    Shi, Guitao
    Chen, Zhenlou
    Bi, Chunjuan
    Wang, Li
    Teng, Jiyan
    Li, Yuansheng
    Xu, Shiyuan
    ATMOSPHERIC ENVIRONMENT, 2011, 45 (03) : 764 - 771
  • [44] Potentially toxic elements in street dust from an urban city of a developing country: ecological and probabilistic health risks assessment
    Kabir, Md. Humayun
    Kormoker, Tapos
    Islam, Md. Saiful
    Khan, Rahat
    Shammi, Rifat Shahid
    Tusher, Tanmoy Roy
    Proshad, Ram
    Islam, Md Shafiqul
    Idris, Abubakr M.
    ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH, 2021, 28 (40) : 57126 - 57148
  • [45] Potentially toxic elements in street dust from an urban city of a developing country: ecological and probabilistic health risks assessment
    Md. Humayun Kabir
    Tapos Kormoker
    Md. Saiful Islam
    Rahat Khan
    Rifat Shahid Shammi
    Tanmoy Roy Tusher
    Ram Proshad
    Md Shafiqul Islam
    Abubakr M. Idris
    Environmental Science and Pollution Research, 2021, 28 : 57126 - 57148
  • [46] Pollution levels and health risk assessment of potential toxic elements in road dust from different functional areas of Plateau city in SW China
    Bo Q.
    Wang J.
    Arabian Journal of Geosciences, 2021, 14 (19)
  • [47] Risk assessment of potentially toxic elements in smaller than 100-μm street dust particles from a valley-city in northwestern China
    Ni Zhao
    Xinwei Lu
    Shigang Chao
    Environmental Geochemistry and Health, 2016, 38 : 483 - 496
  • [48] Risk assessment of potentially toxic elements in smaller than 100-μm street dust particles from a valley-city in northwestern China
    Zhao, Ni
    Lu, Xinwei
    Chao, Shigang
    ENVIRONMENTAL GEOCHEMISTRY AND HEALTH, 2016, 38 (02) : 483 - 496
  • [49] A comprehensive approach to quantify the source identification and human health risk assessment of toxic elements in park dust
    Huang, Chang-Chen
    Cai, Li-Mei
    Xu, Yao-Hui
    Jie, Luo
    Hu, Guo-Cheng
    Chen, Lai-Guo
    Wang, Han-Zhi
    Xu, Xu-Bang
    Mei, Jing-Xian
    ENVIRONMENTAL GEOCHEMISTRY AND HEALTH, 2023, 45 (08) : 5813 - 5827
  • [50] A comprehensive approach to quantify the source identification and human health risk assessment of toxic elements in park dust
    Chang-Chen Huang
    Li-Mei Cai
    Yao-Hui Xu
    Luo Jie
    Guo-Cheng Hu
    Lai-Guo Chen
    Han-Zhi Wang
    Xu-Bang Xu
    Jing-Xian Mei
    Environmental Geochemistry and Health, 2023, 45 : 5813 - 5827