Graphitic carbon nitride-PTD hybrid catalyst for efficient photocatalytic oxidative coupling of arylamine for the production of azoaromatic under visible light

被引：0

作者：

Singh, Nidhi ^{[1
]}

Yadav, Rajesh K. ^{[1
]}

Mishra, Shaifali ^{[1
]}

Shahin, Rehana ^{[1
]}

Singh, Satyam ^{[1
]}

Singhal, Rajat ^{[2
]}

Gupta, Navneet K. ^{[2
]}

Baeg, Jin-OoK ^{[3
]}

Obaidullah, Ahmad J. ^{[4
]}

Yadav, Krishna Kumar ^{[5
,6
]}

Umar, Ahmad ^{[7
,8
,9
]}

Almas, Tubia ^{[7
,8
]}

机构：

[1] Madan Mohan Malaviya Univ Technol, Dept Chem & Environm Sci, Gorakhpur 273010, Uttar Pradesh, India

[2] Indian Inst Sci, Ctr Sustainable Technol, Bangalore Gulmohar Marg, Bengaluru 560012, India

[3] Korea Res Inst Chem Technol, 141 Gajeong Ro, Daejeon, South Korea

[4] King Saud Univ, Coll Pharm, Dept Pharmaceut Chem, POB 2457, Riyadh 11451, Saudi Arabia

[5] Madhyanchal Profess Univ, Fac Sci & Technol, Bhopal 462044, India

[6] Al Ayen Univ, Sci Res Ctr, Environm & Atmospher Sci Res Grp, Nasiriyah 64001, Iraq

[7] Najran Univ, Fac Sci & Arts, Dept Chem, Najran 11001, Saudi Arabia

[8] Najran Univ, PCSED, Najran 11001, Saudi Arabia

[9] Ohio State Univ, Dept Mat Sci & Engn, Columbus, OH 43210 USA

来源：

JOURNAL OF MOLECULAR STRUCTURE | 2024年 / 1318卷

关键词：

G-PTD photocatalyst; Graphitic carbon nitride; Azo; -N=N- group; Dyes; SOLAR FUEL PRODUCTION; HIGHLY EFFICIENT; H-2; EVOLUTION; NANOPARTICLES; SYSTEM;

D O I：

10.1016/j.molstruc.2024.139144

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Oxidative coupling of amine derivatives to selectively synthesize pharmaceutical materials has been realized via photocatalysis. Herein we report on the fabrication and development of a graphitic carbon nitride (G) based visible light active photocatalyst (G-PTD), which is melamine converted graphitic carbon nitride(G) covalently integrated to a light harvesting perylene tetracarboxylic dianhydride (PTD) molecule. The synthesized photocatalyst has various functions in a highly active manner leading to high yield of newly generated azoaromatic compound. The current research endeavour highlights on the fabrication and utilization of a graphitic carbon nitride based photocatalyst for direct oxidative coupling of arylamines.

引用

页数：8

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