Design and Performance of Quantum Dot Light-emitting Diode Based on TiO2 Modified Layer

被引:0
|
作者
Liu W.-W. [1 ]
Kong Y.-C. [1 ]
Chen X.-B. [1 ]
Hu X.-Y. [1 ]
Miao Z.-Z. [1 ]
机构
[1] Department of Physics and Electronic Engineering, Yancheng Teachers University, Yancheng
来源
基金
中国国家自然科学基金;
关键词
Interface modification; Light-emitting diodes; Quantum dot; TiO[!sub]2[!/sub;
D O I
10.37188/CJL.20220002
中图分类号
学科分类号
摘要
Due to high color saturation and high color purity, quantum dot(QD) light-emitting diodes(QLEDs) have become one of the hotspots in LEDs research for their potential application in lighting and display. Surface and interface issues have become a thorny issue which restricting the development of QLEDs with multilayer structure. In this paper, the interface between electron transport layer zinc oxide(ZnO) and QDs emitting layer was modified by inserting titanium dioxide(TiO2) layers with different thickness based on atomic layer deposition(ALD) technology. After inserting 0.270 nm TiO2 modified layer, the leakage current of the QLEDs was significantly reduced about an order of magnitude, and the average lifetime of the excitons increased from 15.94 ns to 16.61 ns, indicating that the insertion of the TiO2 modified layer can effectively prevent the exciton quenching in QDs emitting layer, thereby enhancing the current efficiency of the QLEDs under low driving voltage(about increased 15%). The above results are expected to provide a reference for the industrialization of QLEDs in the field of lighting and display. © 2022, Science Press. All right reserved.
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页码:381 / 387
页数:6
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共 34 条
  • [1] MOON H, LEE C, LEE W, Et al., Stability of quantum dots, quantum dot films, and quantum dot light-emitting diodes for display applications, Adv. Mater, 31, 34, (2019)
  • [2] HUANG Y G, HSIANG E L, DENG M Y, Et al., Mini-LED, Micro-LED and OLED displays: present status and future perspectives, Light: Sci. Appl, 9, (2020)
  • [3] SUN Y Z, JIANG Y B, SUN X W, Et al., Beyond OLED: efficient quantum dot light-emitting diodes for display and lighting application, Chem. Rec, 19, 8, pp. 1729-1752, (2019)
  • [4] ZHAO Y, GAO X P, LU P, Et al., Quantum dot-based white LEDs and their applications of SMART lighting, Chin. J. Liq. Cryst. Disp, 36, 1, pp. 187-202, (2021)
  • [5] SONG J J, WANG O Y, SHEN H B, Et al., Over 30% external quantum efficiency light-emitting diodes by engineering quantum dot-assisted energy level match for hole transport layer, Adv. Funct. Mater, 29, 33, (2019)
  • [6] FU Y, JIANG W, KIM D, Et al., Highly efficient and fully solution-processed inverted light-emitting diodes with charge control interlayers, ACS Appl. Mater. Interfaces, 10, 20, pp. 17295-17300, (2018)
  • [7] ZHANG H, SU Q, SUN Y Z, Et al., Efficient and color stable white quantum-dot light-emitting diodes with external quantum efficiency over 23%, Adv. Opt. Mater, 6, 16, (2018)
  • [8] DONG J Y, NG K W, SONG Y M, Et al., Observation and suppression of stacking interface states in sandwich-structured quantum dot light-emitting diodes, ACS Appl. Mater. Interfaces, 13, 47, pp. 56630-56637, (2021)
  • [9] ZHANG H, SU Q, CHEN S M., Suppressing Förster resonance energy transfer in close-packed quantum-dot thin film: toward efficient quantum-dot light-emitting diodes with external quantum efficiency over 21.6%, Adv. Opt. Mater, 8, 10, (2020)
  • [10] TIAN F Q, ZHU Y B, XU Z W, Et al., Achieving highly efficient and stable quantum dot light-emitting diodes with interface modification, IEEE Electron Device Lett, 41, 9, pp. 1384-1387, (2020)