Gas-liquid countercurrent flow characteristics in a microbubble column reactor

被引:0
|
作者
Chang, Yu [1 ]
Shang, Qichen [1 ]
Sheng, Lin [1 ]
Deng, Jian [1 ]
Luo, Guangsheng [1 ]
机构
[1] Tsinghua Univ, Dept Chem Engn, State Key Lab Chem Engn, Beijing 100084, Peoples R China
基金
中国国家自然科学基金;
关键词
Microdispersion; Countercurrent flow; Microbubble column reactor; MASS;
D O I
10.1016/j.ces.2024.120573
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Countercurrent flow mode is widely utilized in many chemical unit operations due to its effective enhancement of mass transfer driving force. While the microbubble column reactor has garnered attention for its substantial gas-liquid specific surface area and fast mass transfer rate under the concurrent flow condition, countercurrent flow microbubble column reactors remain relatively underexplored. Consequently, in this study a novel microbubble generator device featuring gas-liquid co-crossing a microfiltration membrane was developed. This device could generate microbubbles with narrow size distribution, and proved suitable for integration into the countercurrent microbubble column reactor. Further investigation ensued to elucidate the operational principles of this dispersion method. Finally, the hydrodynamic behavior of the countercurrent microbubble column reactor was examined. Remarkably, a gas-liquid-specific surface area 2300 m2/m3 2 /m 3 was reached, surpassing that of conventional bubble column reactors by a significant margin. New gas-liquid chemical processes and process intensification technologies could be developed accordingly.
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页数:11
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