Mixed rare earth metals production from surface soil in Idaho, USA: Techno-economic analysis and greenhouse gas emission assessment
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作者:
Browna, Rebecca M.
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Univ Idaho, Environm Sci Program, Idaho Falls, ID 83402 USA
Idaho Natl Lab, Dept Mat Recovery & Recycling, Idaho Falls, ID 83402 USA
Univ Idaho, Tingey Adm Bldg,Suite 312, Idaho Falls, ID 83402 USAUniv Idaho, Environm Sci Program, Idaho Falls, ID 83402 USA
Browna, Rebecca M.
[1
,2
,5
]
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Struhs, Ethan
[3
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Mirkoueia, Amin
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机构:
Univ Idaho, Environm Sci Program, Idaho Falls, ID 83402 USA
Univ Idaho, Dept Mech Engn, Idaho Falls, ID 83402 USA
Univ Idaho, Dept Nucl Engn & Ind Management, Idaho Falls, ID 83402 USA
Univ Idaho, Tingey Adm Bldg,Suite 312, Idaho Falls, ID 83402 USAUniv Idaho, Environm Sci Program, Idaho Falls, ID 83402 USA
Mirkoueia, Amin
[1
,3
,4
,5
]
Raja, Krishnan
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机构:
Univ Idaho, Dept Nucl Engn & Ind Management, Idaho Falls, ID 83402 USAUniv Idaho, Environm Sci Program, Idaho Falls, ID 83402 USA
Raja, Krishnan
[4
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Reed, David
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机构:
Idaho Natl Lab, Dept Mat Recovery & Recycling, Idaho Falls, ID 83402 USAUniv Idaho, Environm Sci Program, Idaho Falls, ID 83402 USA
Reed, David
[2
]
机构:
[1] Univ Idaho, Environm Sci Program, Idaho Falls, ID 83402 USA
[2] Idaho Natl Lab, Dept Mat Recovery & Recycling, Idaho Falls, ID 83402 USA
[3] Univ Idaho, Dept Mech Engn, Idaho Falls, ID 83402 USA
[4] Univ Idaho, Dept Nucl Engn & Ind Management, Idaho Falls, ID 83402 USA
[5] Univ Idaho, Tingey Adm Bldg,Suite 312, Idaho Falls, ID 83402 USA
Rare earth elements;
Rare earth metals;
Life cycle assessment;
Techno-economic assessment;
Bio-organic acid leaching;
Molten salt electrolysis;
ELEMENTS;
RESOURCES;
D O I:
10.1016/j.scitotenv.2024.173945
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
Rare earth elements are crucial for the development of cutting-edge technologies in various sectors, such as energy, transportation, and health care. Traditional extraction of rare earth elements from soil and ore deposits primarily involves chemical leaching and solvent extraction. Environmental-based biological rare earth element extraction, such as bioleaching, can be a promising alternative to mitigate pollution and hazardous wastes. We investigated the sustainability aspects (techno-economic and environmental impact) of mixed rare earth metals production from soil in Idaho, USA. We focused on the bioleaching of surface soil using techno-economic analysis and "cradle-to-gate" life cycle assessment. The system boundary included collection, transportation, bioleaching, and molten salt electrolysis. Our results revealed that the mixed rare earth metals (including Nd, Ce, and La) production costs approximately $10,851 per metric ton and generates 1.9 x106 kg CO2 eq./ton. Our results showed that most emissions are due to energy consumption during bioleaching. Over a 100-year time horizon ultrasound-assisted bioleaching can reduce greenhouse gas emissions by approximately 91 % compared to the traditional bioleaching process by decreasing the organic acid leaching process time and energy consumption. Our work demonstrates that higher solids loading in leaching with biological reactions can promote economic feasibility and reduce chemical wastes
机构:
Xi'an Key Laboratory of C1 Compound Bioconversion Technology, School of Chemical Engineering and Technology, Xi'an Jiaotong University, Xi'an,710049, ChinaXi'an Key Laboratory of C1 Compound Bioconversion Technology, School of Chemical Engineering and Technology, Xi'an Jiaotong University, Xi'an,710049, China
Zhang, Chenyue
Fu, Rongzhan
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机构:
Shaanxi Key Laboratory of Degradable Biomedical Materials, School of Chemical Engineering, Northwest University, Xi'an,710069, ChinaXi'an Key Laboratory of C1 Compound Bioconversion Technology, School of Chemical Engineering and Technology, Xi'an Jiaotong University, Xi'an,710049, China
Fu, Rongzhan
Kang, Lixia
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机构:
Xi'an Key Laboratory of C1 Compound Bioconversion Technology, School of Chemical Engineering and Technology, Xi'an Jiaotong University, Xi'an,710049, ChinaXi'an Key Laboratory of C1 Compound Bioconversion Technology, School of Chemical Engineering and Technology, Xi'an Jiaotong University, Xi'an,710049, China
Kang, Lixia
Ma, Yingqun
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机构:
Xi'an Key Laboratory of C1 Compound Bioconversion Technology, School of Chemical Engineering and Technology, Xi'an Jiaotong University, Xi'an,710049, ChinaXi'an Key Laboratory of C1 Compound Bioconversion Technology, School of Chemical Engineering and Technology, Xi'an Jiaotong University, Xi'an,710049, China
Ma, Yingqun
Fan, Daidi
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机构:
Shaanxi Key Laboratory of Degradable Biomedical Materials, School of Chemical Engineering, Northwest University, Xi'an,710069, ChinaXi'an Key Laboratory of C1 Compound Bioconversion Technology, School of Chemical Engineering and Technology, Xi'an Jiaotong University, Xi'an,710049, China
Fan, Daidi
Fei, Qiang
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机构:
Xi'an Key Laboratory of C1 Compound Bioconversion Technology, School of Chemical Engineering and Technology, Xi'an Jiaotong University, Xi'an,710049, ChinaXi'an Key Laboratory of C1 Compound Bioconversion Technology, School of Chemical Engineering and Technology, Xi'an Jiaotong University, Xi'an,710049, China
机构:
Univ Groningen, Integrated Res Energy Environm & Soc, Nijenborgh 6,, NL-9747 AG Groningen, NetherlandsUniv Groningen, Integrated Res Energy Environm & Soc, Nijenborgh 6,, NL-9747 AG Groningen, Netherlands
Yang, Fan
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机构:
Meerman, Hans
Zhang, Zhenhua
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机构:
Univ Groningen, Univ Med Ctr Groningen, Genom Coordinat Ctr, Antonius Deusinglaan 1,, NL-9713 AV Groningen, Netherlands
Univ Groningen, Univ Med Ctr Groningen, Dept Genet, Antonius Deusinglaan 1, NL-9713 AV Groningen, NetherlandsUniv Groningen, Integrated Res Energy Environm & Soc, Nijenborgh 6,, NL-9747 AG Groningen, Netherlands
Zhang, Zhenhua
Jiang, Jianrong
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机构:
Xi An Jiao Tong Univ, Sch Chem Engn & Technol, Shaanxi Key Lab Energy Chem Proc Intensificat, Xian 710049, Shaanxi, Peoples R ChinaUniv Groningen, Integrated Res Energy Environm & Soc, Nijenborgh 6,, NL-9747 AG Groningen, Netherlands
Jiang, Jianrong
Faaij, Andre
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Univ Groningen, Integrated Res Energy Environm & Soc, Nijenborgh 6,, NL-9747 AG Groningen, Netherlands
TNO Energy Transit, Princetonlaan 6, NL-3584 CB Utrecht, NetherlandsUniv Groningen, Integrated Res Energy Environm & Soc, Nijenborgh 6,, NL-9747 AG Groningen, Netherlands