Treefrog-Inspired Flexible Electrode with High Permeability, Stable Adhesion, and Robust Durability

Long-term continuous monitoring (LTCM) of physiological electrical signals is an effective means for detecting several cardiovascular diseases. However, the integrated challenges of stable adhesion, low impedance, and robust durability under different skin conditions significantly hinder the application of flexible electrodes in LTCM. This paper proposes a structured electrode inspired by the treefrog web, comprising dispersed pillars at the bottom and asymmetric cone holes at the top. Attachment structures with a dispersed pillar improve the contact stability (adhesion increases 2.79/13.16 times in dry/wet conditions compared to an electrode without structure). Improved permeable duct structure provides high permeability (12 times compared to cotton). Due to high adhesion and permeability, the electrode's durability is 40 times larger than commercial Ag/AgCl electrodes. The treefrog web-like electrode has great advantages in permeability, adhesion, and durability, resulting in prospects for application in physiological electrical signal detection and a new design idea for LTCM wearable dry electrodes. The challenges of instable adhesion, low impedance, and robust durability that hinder the long-term application of in vitro bioelectrodes. Inspired by treefrog web and bird's beak, through the optimization design, a web-like electrode, which can solve these complex integrated challenges, is proposed. Proposed electrode has the most balanced mechanical, electrical, and electrode properties of typical electrodes reported in recent years. image