Preparation of colored TiO 2 flower/Ti 3 C 2 for efficient photocatalytic degradation of tetracycline

被引:6
|
作者
Deng, Quanhao [1 ,2 ]
Yu, Leyang [1 ,2 ]
Chen, Qianmei [1 ,2 ]
Wen, Jianfeng [1 ,2 ]
Zhang, Anqi [1 ,2 ]
Li, Ming [1 ,2 ]
Tang, Tao [1 ,2 ]
Hu, Guanghui [1 ,2 ]
Jiang, Li [1 ,2 ]
Cao, Xueli [1 ,2 ]
Yao, Yi [2 ,3 ]
机构
[1] Guilin Univ Technol, Coll Phys & Elect Informat Engn, Guilin 541004, Peoples R China
[2] Guilin Univ Technol, Educ Dept Guangxi Zhuang Autonomous Reg, Key Lab Low dimens Struct Phys & Applicat, Guilin 541004, Peoples R China
[3] Guilin Univ Technol, Coll Environm Sci & Engn, Guangxi Collaborat Innovat Ctr Water Pollut Contro, 319 Yanshan St, Guilin 541004, Peoples R China
关键词
ColoredTiO2; Oxygen vacancy; Photocatalysis; NaHB4; STEP HYDROTHERMAL SYNTHESIS; VISIBLE-LIGHT; HYDROGEN-PRODUCTION; CHARGE-TRANSFER; DOPED TIO2; WATER; ANTIBIOTICS; NANOCOMPOSITE; OXIDATION; COMPOSITE;
D O I
10.1016/j.inoche.2024.112317
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
Herein, colored TiO 2 flowers grown on Ti 3 C 2 (XTFT, where X = 250 degrees C, 300 degrees C, and 350 degrees C representing heating temperature) are prepared as photocatalysts for degradation of tetracycline using hydrothermal method and CVD process. TiO 2 has a suitable bandgap as a photocatalyst. However, in practical applications, TiO 2 cannot effectively utilize visible light and the recombination of photogenerated carriers is excessively fast. The fabrication of XTFT through defect engineering compensates for the shortcomings of pure TiO 2 in photocatalytic applications, following which the bandgap of TiO 2 is reduced and the TiO 2 surface becomes discolored and effectively responds to visible light. Ti 3 C 2 , a promising auxiliary material in the field of photocatalysis, is used as a photocatalyst in the degradation of tetracycline via defect engineering. After forming a composite with TiO 2 , Ti 3 C 2 can effectively separate TiO 2 photogenerated carriers to enhance the photocatalytic performance of TiO 2 . The degradation rate of 50 mL 50 mg/L tetracycline by 50 mg 300TFT under visible light irradiation for 30 min is 96.3 %. Compared with pure TiO 2 , the photocatalytic efficiency is significantly improved, thus providing a new idea for realization of highly efficient visible photocatalysis in the field of environmental pollution in future.
引用
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页数:10
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